# Electronic Supplementary Material (ESI) for Physical Chemistry Chemical Physics. # This journal is © the Owner Societies 2023 ####################################################################### # # This file contains crystal structure data downloaded from the # Cambridge Structural Database (CSD) hosted by the Cambridge # Crystallographic Data Centre (CCDC). # # Full information about CCDC data access policies and citation # guidelines are available at http://www.ccdc.cam.ac.uk/access/V1 # # Audit and citation data items may have been added by the CCDC. # Please retain this information to preserve the provenance of # this file and to allow appropriate attribution of the data. # ####################################################################### data_Npe-TCNQ _database_code_depnum_ccdc_archive 'CCDC 2286627' loop_ _audit_author_name _audit_author_address 'Joseph E. Reynolds III' ;Sandia National laboratory United States of America ; _audit_update_record ; 2023-08-03 deposited with the CCDC. 2023-09-26 downloaded from the CCDC. ; _audit_creation_date 2022-06-28 _audit_creation_method ; Olex2 1.5 (compiled 2021.12.09 svn.r5202d8cf for OlexSys, GUI svn.r6439) ; _shelx_SHELXL_version_number 2018/3 _chemical_name_common ? _chemical_name_systematic 3TCNQ2NPE _chemical_formula_moiety 'C17 H13 N, 1.5(C12 H4 N4)' _chemical_formula_sum 'C35 H19 N7' _chemical_formula_weight 537.57 _chemical_melting_point ? _chemical_oxdiff_formula N4C18H18 _chemical_oxdiff_usercomment 'Solvent MeCN. 1:1 NVP:TCNQ' loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0181 0.0091 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0311 0.0180 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _space_group_crystal_system triclinic _space_group_IT_number 2 _space_group_name_H-M_alt 'P -1' _space_group_name_Hall '-P 1' loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, -y, -z' _cell_length_a 9.8862(4) _cell_length_b 11.8127(5) _cell_length_c 12.3102(5) _cell_angle_alpha 93.827(3) _cell_angle_beta 93.940(3) _cell_angle_gamma 111.868(4) _cell_volume 1324.40(9) _cell_formula_units_Z 2 _cell_measurement_reflns_used 9179 _cell_measurement_temperature 102(3) _cell_measurement_theta_max 72.7970 _cell_measurement_theta_min 3.5720 _shelx_estimated_absorpt_T_max 0.972 _shelx_estimated_absorpt_T_min 0.769 _exptl_absorpt_coefficient_mu 0.660 _exptl_absorpt_correction_T_max 1.000 _exptl_absorpt_correction_T_min 0.628 _exptl_absorpt_correction_type gaussian _exptl_absorpt_process_details ; CrysAlisPro 1.171.41.93a (Rigaku Oxford Diffraction, 2020) Numerical absorption correction based on gaussian integration over a multifaceted crystal model Empirical absorption correction using spherical harmonics, implemented in SCALE3 ABSPACK scaling algorithm. ; _exptl_absorpt_special_details ? _exptl_crystal_colour 'clear dark blue' _exptl_crystal_colour_lustre clear _exptl_crystal_colour_modifier dark _exptl_crystal_colour_primary blue _exptl_crystal_density_diffrn 1.348 _exptl_crystal_density_meas ? _exptl_crystal_density_method ? _exptl_crystal_description prism _exptl_crystal_F_000 556 loop_ _exptl_crystal_face_index_h _exptl_crystal_face_index_k _exptl_crystal_face_index_l _exptl_crystal_face_perp_dist 2 4 5 0.0682 -6 3 3 0.2140 -6 0 -1 0.1597 -3 -3 -5 0.1035 -6 1 0 0.1633 4 -5 -6 0.1346 6 -2 0 0.2000 0 5 -6 0.0197 0 -5 6 0.0214 _exptl_crystal_preparation ? _exptl_crystal_recrystallization_method '1:1 (DMF/MeCN)' _exptl_crystal_size_max 0.421 _exptl_crystal_size_mid 0.186 _exptl_crystal_size_min 0.044 loop_ _exptl_oxdiff_crystal_face_indexfrac_h _exptl_oxdiff_crystal_face_indexfrac_k _exptl_oxdiff_crystal_face_indexfrac_l _exptl_oxdiff_crystal_face_x _exptl_oxdiff_crystal_face_y _exptl_oxdiff_crystal_face_z 1.9140 3.9586 4.6439 -0.5221 0.7533 0.4000 -6.1293 3.3378 2.7052 -0.2046 0.3045 -0.9303 -5.8139 -0.0079 -0.9175 0.1778 -0.2496 -0.9519 -2.6530 -3.0482 -4.7727 0.5621 -0.6596 -0.4990 -6.1226 0.7714 -0.2092 0.1080 -0.1334 -0.9852 3.7482 -4.5790 -5.5566 0.5595 -0.6489 0.5156 6.3939 -2.4375 -0.0922 -0.1033 -0.0949 0.9901 -0.3466 4.8916 -6.4030 0.8754 0.4777 0.0739 0.2698 -4.8636 6.4102 -0.8749 -0.4766 -0.0858 _exptl_transmission_factor_max ? _exptl_transmission_factor_min ? _diffrn_reflns_av_R_equivalents 0.0235 _diffrn_reflns_av_unetI/netI 0.0209 _diffrn_reflns_Laue_measured_fraction_full 1.000 _diffrn_reflns_Laue_measured_fraction_max 0.972 _diffrn_reflns_limit_h_max 12 _diffrn_reflns_limit_h_min -9 _diffrn_reflns_limit_k_max 14 _diffrn_reflns_limit_k_min -14 _diffrn_reflns_limit_l_max 15 _diffrn_reflns_limit_l_min -15 _diffrn_reflns_number 14402 _diffrn_reflns_point_group_measured_fraction_full 1.000 _diffrn_reflns_point_group_measured_fraction_max 0.972 _diffrn_reflns_theta_full 67.684 _diffrn_reflns_theta_max 73.000 _diffrn_reflns_theta_min 3.617 _diffrn_ambient_environment N~2~ _diffrn_ambient_temperature 102(3) _diffrn_detector 'CCD plate' _diffrn_detector_area_resol_mean 10.2358 _diffrn_detector_type Atlas _diffrn_measured_fraction_theta_full 1.000 _diffrn_measured_fraction_theta_max 0.972 _diffrn_measurement_details ; List of Runs (angles in degrees, time in seconds): # Type Start End Width t~exp~ \w \q \k \f Frames #-------------------------------------------------------------------------- 1 \w -117.00 -18.00 1.00 2.50 -- -42.59 -38.00 90.00 99 2 \w -87.00 -6.00 1.00 2.50 -- -42.59 125.00-120.00 81 3 \w -123.00 -2.00 1.00 2.50 -- -42.59 -19.00 150.00 121 4 \w 27.00 99.00 1.00 2.50 -- 42.59-125.00 60.00 72 5 \w 27.00 99.00 1.00 2.50 -- 42.59-125.00 0.00 72 6 \w 31.00 130.00 1.00 7.50 -- 104.03 -45.00-150.00 99 7 \w 78.00 177.00 1.00 7.50 -- 104.03 45.00-120.00 99 8 \w 103.00 178.00 1.00 7.50 -- 104.03 77.00 -90.00 75 9 \w 31.00 112.00 1.00 7.50 -- 104.03-125.00 -30.00 81 10 \w 22.00 106.00 1.00 7.50 -- 104.03 -95.00 60.00 84 11 \w 78.00 177.00 1.00 7.50 -- 104.03 45.00 -30.00 99 12 \w 78.00 177.00 1.00 7.50 -- 104.03 45.00-180.00 99 13 \w 22.00 106.00 1.00 7.50 -- 104.03 -95.00 120.00 84 14 \w 22.00 106.00 1.00 7.50 -- 104.03 -95.00 0.00 84 15 \w 28.00 137.00 1.00 7.50 -- 104.03 -77.00-180.00 109 16 \w 28.00 132.00 1.00 7.50 -- 104.03 -30.00 -60.00 104 17 \w -116.00 -14.00 1.00 2.50 -- -42.59 -57.00 60.00 102 18 \w -116.00 -14.00 1.00 2.50 -- -42.59 -57.00 -30.00 102 19 \w 14.00 116.00 1.00 2.50 -- 42.59 57.00 -60.00 102 ; _diffrn_measurement_device 'four-circle diffractometer' _diffrn_measurement_device_type 'SuperNova, Dual, Cu at home/near, Atlas' _diffrn_measurement_method '\w scans' _diffrn_orient_matrix_type 'CrysAlisPro convention (1999,Acta A55,543-557)' _diffrn_orient_matrix_UB_11 -0.0112428000 _diffrn_orient_matrix_UB_12 0.0175216000 _diffrn_orient_matrix_UB_13 -0.1227225000 _diffrn_orient_matrix_UB_21 0.0382017000 _diffrn_orient_matrix_UB_22 0.1380527000 _diffrn_orient_matrix_UB_23 0.0287893000 _diffrn_orient_matrix_UB_31 0.1640097000 _diffrn_orient_matrix_UB_32 0.0240970000 _diffrn_orient_matrix_UB_33 -0.0020083000 _diffrn_radiation_monochromator mirror _diffrn_radiation_probe x-ray _diffrn_radiation_type 'Cu K\a' _diffrn_radiation_wavelength 1.54184 _diffrn_source 'micro-focus sealed X-ray tube' _diffrn_source_type 'SuperNova (Cu) X-ray Source' _reflns_Friedel_coverage 0.000 _reflns_Friedel_fraction_full . _reflns_Friedel_fraction_max . _reflns_number_gt 4451 _reflns_number_total 5154 _reflns_special_details ; Reflections were merged by SHELXL according to the crystal class for the calculation of statistics and refinement. _reflns_Friedel_fraction is defined as the number of unique Friedel pairs measured divided by the number that would be possible theoretically, ignoring centric projections and systematic absences. ; _reflns_threshold_expression 'I > 2\s(I)' _computing_cell_refinement 'CrysAlisPro 1.171.41.93a (Rigaku OD, 2020)' _computing_data_collection 'CrysAlisPro 1.171.41.93a (Rigaku OD, 2020)' _computing_data_reduction 'CrysAlisPro 1.171.41.93a (Rigaku OD, 2020)' _computing_molecular_graphics 'Olex2 1.5 (Dolomanov et al., 2009)' _computing_publication_material 'Olex2 1.5 (Dolomanov et al., 2009)' _computing_structure_refinement 'SHELXL 2018/3 (Sheldrick, 2015)' _computing_structure_solution 'SHELXS (Sheldrick, 2008)' _refine_diff_density_max 0.274 _refine_diff_density_min -0.195 _refine_diff_density_rms 0.043 _refine_ls_extinction_coef . _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.031 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 379 _refine_ls_number_reflns 5154 _refine_ls_number_restraints 0 _refine_ls_R_factor_all 0.0431 _refine_ls_R_factor_gt 0.0372 _refine_ls_restrained_S_all 1.031 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.0650P)^2^+0.1666P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.1021 _refine_ls_wR_factor_ref 0.1073 _refine_special_details ? _olex2_refinement_description ; 1. Fixed Uiso At 1.2 times of: All C(H) groups 2.a Aromatic/amide H refined with riding coordinates: C1(H1), C2(H2), C4(H4), C5(H5), C6(H6), C7(H7), C9(H9), C10(H10), C11(H11), C13(H13), C14(H14), C15(H15), C16(H16), C22(H22), C23(H23), C25(H25), C26(H26), C34(H34), C35(H35) ; _atom_sites_solution_hydrogens geom _atom_sites_solution_primary direct _atom_sites_solution_secondary ? loop_ _atom_site_label _atom_site_type_symbol _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_occupancy _atom_site_site_symmetry_order _atom_site_calc_flag _atom_site_refinement_flags_posn _atom_site_refinement_flags_adp _atom_site_refinement_flags_occupancy _atom_site_disorder_assembly _atom_site_disorder_group N1 N 0.17548(11) 0.28132(9) 0.51408(8) 0.0242(2) Uani 1 1 d . . . . . C1 C 0.11944(13) 0.36792(11) 0.50650(10) 0.0257(3) Uani 1 1 d . . . . . H1 H 0.034055 0.358667 0.541900 0.031 Uiso 1 1 calc R U . . . C2 C 0.17803(13) 0.47030(11) 0.45028(10) 0.0248(2) Uani 1 1 d . . . . . H2 H 0.131912 0.527785 0.446903 0.030 Uiso 1 1 calc R U . . . C3 C 0.30503(12) 0.48883(10) 0.39859(9) 0.0214(2) Uani 1 1 d . . . . . C4 C 0.36365(12) 0.39816(10) 0.40551(9) 0.0233(2) Uani 1 1 d . . . . . H4 H 0.449089 0.404840 0.371155 0.028 Uiso 1 1 calc R U . . . C5 C 0.29623(12) 0.29879(10) 0.46275(9) 0.0230(2) Uani 1 1 d . . . . . H5 H 0.338279 0.238556 0.466013 0.028 Uiso 1 1 calc R U . . . C6 C 0.36807(12) 0.59846(10) 0.34144(9) 0.0233(2) Uani 1 1 d . . . . . H6 H 0.311646 0.647548 0.331841 0.028 Uiso 1 1 calc R U . . . C7 C 0.49860(12) 0.63543(10) 0.30153(9) 0.0209(2) Uani 1 1 d . . . . . H7 H 0.556571 0.588129 0.314112 0.025 Uiso 1 1 calc R U . . . C8 C 0.56051(12) 0.74260(10) 0.23997(9) 0.0201(2) Uani 1 1 d . . . . . C9 C 0.49245(13) 0.82551(10) 0.23026(9) 0.0235(2) Uani 1 1 d . . . . . H9 H 0.411472 0.817679 0.270660 0.028 Uiso 1 1 calc R U . . . C10 C 0.53999(13) 0.92080(10) 0.16229(10) 0.0249(2) Uani 1 1 d . . . . . H10 H 0.491486 0.976511 0.157705 0.030 Uiso 1 1 calc R U . . . C11 C 0.65578(13) 0.93381(10) 0.10267(9) 0.0238(2) Uani 1 1 d . . . . . H11 H 0.684685 0.996401 0.054619 0.029 Uiso 1 1 calc R U . . . C12 C 0.73256(12) 0.85467(10) 0.11219(9) 0.0207(2) Uani 1 1 d . . . . . C13 C 0.85430(13) 0.86905(10) 0.05228(9) 0.0245(2) Uani 1 1 d . . . . . H13 H 0.882111 0.931018 0.003559 0.029 Uiso 1 1 calc R U . . . C14 C 0.93277(13) 0.79556(11) 0.06306(10) 0.0265(3) Uani 1 1 d . . . . . H14 H 1.013853 0.806153 0.022041 0.032 Uiso 1 1 calc R U . . . C15 C 0.89173(13) 0.70391(10) 0.13583(9) 0.0241(2) Uani 1 1 d . . . . . H15 H 0.947368 0.654118 0.144970 0.029 Uiso 1 1 calc R U . . . C16 C 0.77289(12) 0.68563(10) 0.19350(9) 0.0213(2) Uani 1 1 d . . . . . H16 H 0.746817 0.622579 0.241222 0.026 Uiso 1 1 calc R U . . . C17 C 0.68776(12) 0.75917(9) 0.18335(9) 0.0191(2) Uani 1 1 d . . . . . N2 N 0.36223(12) 0.13406(10) 0.18972(9) 0.0302(2) Uani 1 1 d . . . . . N3 N 0.16050(11) -0.18151(9) 0.36785(8) 0.0267(2) Uani 1 1 d . . . . . N4 N -0.51495(12) 0.10923(10) 0.45992(9) 0.0330(3) Uani 1 1 d . . . . . N5 N -0.28285(12) 0.40113(9) 0.27771(9) 0.0305(2) Uani 1 1 d . . . . . C18 C 0.26447(13) 0.07817(11) 0.23461(9) 0.0226(2) Uani 1 1 d . . . . . C19 C 0.14831(12) -0.09675(10) 0.33519(9) 0.0212(2) Uani 1 1 d . . . . . C20 C 0.14174(12) 0.01107(10) 0.29172(9) 0.0200(2) Uani 1 1 d . . . . . C21 C 0.03000(12) 0.05244(10) 0.30371(8) 0.0190(2) Uani 1 1 d . . . . . C22 C -0.09200(12) -0.00973(10) 0.36492(9) 0.0189(2) Uani 1 1 d . . . . . H22 H -0.099194 -0.083821 0.394407 0.023 Uiso 1 1 calc R U . . . C23 C -0.19546(12) 0.03712(10) 0.38023(8) 0.0190(2) Uani 1 1 d . . . . . H23 H -0.274325 -0.004066 0.421154 0.023 Uiso 1 1 calc R U . . . C24 C -0.18804(12) 0.14935(10) 0.33515(8) 0.0186(2) Uani 1 1 d . . . . . C25 C -0.06912(12) 0.20837(10) 0.27054(9) 0.0200(2) Uani 1 1 d . . . . . H25 H -0.063831 0.280694 0.238521 0.024 Uiso 1 1 calc R U . . . C26 C 0.03365(12) 0.16189(10) 0.25548(9) 0.0203(2) Uani 1 1 d . . . . . H26 H 0.110446 0.201556 0.212279 0.024 Uiso 1 1 calc R U . . . C27 C -0.29025(12) 0.20007(10) 0.35240(9) 0.0200(2) Uani 1 1 d . . . . . C28 C -0.41285(13) 0.14682(10) 0.41351(9) 0.0232(2) Uani 1 1 d . . . . . C29 C -0.28395(12) 0.31196(10) 0.30923(9) 0.0223(2) Uani 1 1 d . . . . . N6 N 0.06213(11) 0.46879(10) 0.14545(9) 0.0310(2) Uani 1 1 d . . . . . N7 N 0.25844(12) 0.77467(9) -0.04490(9) 0.0301(2) Uani 1 1 d . . . . . C30 C 0.15714(13) 0.51934(10) 0.09602(9) 0.0230(2) Uani 1 1 d . . . . . C31 C 0.26624(12) 0.68883(10) -0.01156(9) 0.0218(2) Uani 1 1 d . . . . . C32 C 0.27434(12) 0.58219(10) 0.03292(9) 0.0201(2) Uani 1 1 d . . . . . C33 C 0.38631(12) 0.54224(9) 0.01707(8) 0.0186(2) Uani 1 1 d . . . . . C34 C 0.50019(12) 0.60442(10) -0.05069(9) 0.0199(2) Uani 1 1 d . . . . . H34 H 0.498944 0.674544 -0.083626 0.024 Uiso 1 1 calc R U . . . C35 C 0.39249(12) 0.43670(9) 0.06712(9) 0.0198(2) Uani 1 1 d . . . . . H35 H 0.319180 0.395668 0.112512 0.024 Uiso 1 1 calc R U . . . loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_23 _atom_site_aniso_U_13 _atom_site_aniso_U_12 N1 0.0248(5) 0.0242(5) 0.0242(5) 0.0043(4) 0.0019(4) 0.0099(4) C1 0.0248(6) 0.0267(6) 0.0279(6) 0.0049(5) 0.0073(5) 0.0114(5) C2 0.0245(6) 0.0242(6) 0.0296(6) 0.0048(5) 0.0061(5) 0.0126(5) C3 0.0196(5) 0.0225(5) 0.0218(5) 0.0017(4) 0.0006(4) 0.0079(4) C4 0.0203(6) 0.0237(6) 0.0266(6) 0.0024(4) 0.0027(4) 0.0092(5) C5 0.0221(6) 0.0220(6) 0.0261(5) 0.0022(4) 0.0001(4) 0.0100(5) C6 0.0235(6) 0.0229(6) 0.0253(5) 0.0038(4) 0.0023(4) 0.0107(5) C7 0.0220(6) 0.0200(5) 0.0214(5) 0.0018(4) 0.0008(4) 0.0090(4) C8 0.0206(5) 0.0178(5) 0.0215(5) 0.0002(4) -0.0007(4) 0.0075(4) C9 0.0217(6) 0.0211(5) 0.0282(6) 0.0010(4) 0.0020(4) 0.0091(4) C10 0.0265(6) 0.0191(5) 0.0317(6) 0.0010(4) -0.0017(5) 0.0127(5) C11 0.0278(6) 0.0169(5) 0.0256(5) 0.0035(4) -0.0018(4) 0.0078(4) C12 0.0215(5) 0.0166(5) 0.0219(5) 0.0009(4) -0.0011(4) 0.0054(4) C13 0.0242(6) 0.0214(5) 0.0246(5) 0.0036(4) 0.0018(4) 0.0046(4) C14 0.0219(6) 0.0280(6) 0.0280(6) -0.0004(5) 0.0044(5) 0.0078(5) C15 0.0232(6) 0.0234(6) 0.0275(6) -0.0002(4) 0.0003(4) 0.0116(5) C16 0.0228(6) 0.0183(5) 0.0231(5) 0.0016(4) -0.0004(4) 0.0087(4) C17 0.0204(5) 0.0158(5) 0.0197(5) 0.0005(4) -0.0005(4) 0.0058(4) N2 0.0279(5) 0.0349(6) 0.0343(6) 0.0121(4) 0.0104(4) 0.0168(5) N3 0.0237(5) 0.0270(5) 0.0340(5) 0.0078(4) 0.0061(4) 0.0135(4) N4 0.0308(6) 0.0353(6) 0.0447(6) 0.0194(5) 0.0161(5) 0.0214(5) N5 0.0360(6) 0.0253(5) 0.0354(6) 0.0082(4) 0.0052(5) 0.0166(4) C18 0.0231(6) 0.0267(6) 0.0229(5) 0.0048(4) 0.0033(4) 0.0144(5) C19 0.0166(5) 0.0261(6) 0.0228(5) 0.0021(4) 0.0040(4) 0.0099(4) C20 0.0196(5) 0.0215(5) 0.0198(5) 0.0022(4) 0.0013(4) 0.0089(4) C21 0.0185(5) 0.0202(5) 0.0176(5) 0.0009(4) 0.0000(4) 0.0071(4) C22 0.0196(5) 0.0174(5) 0.0198(5) 0.0037(4) 0.0007(4) 0.0072(4) C23 0.0187(5) 0.0191(5) 0.0188(5) 0.0036(4) 0.0019(4) 0.0066(4) C24 0.0186(5) 0.0194(5) 0.0178(5) 0.0018(4) -0.0008(4) 0.0078(4) C25 0.0200(5) 0.0201(5) 0.0206(5) 0.0053(4) 0.0022(4) 0.0077(4) C26 0.0189(5) 0.0213(5) 0.0210(5) 0.0060(4) 0.0037(4) 0.0072(4) C27 0.0202(5) 0.0207(5) 0.0207(5) 0.0042(4) 0.0027(4) 0.0091(4) C28 0.0247(6) 0.0239(6) 0.0279(6) 0.0083(5) 0.0046(5) 0.0157(5) C29 0.0214(6) 0.0236(6) 0.0248(5) 0.0033(4) 0.0038(4) 0.0116(5) N6 0.0263(5) 0.0315(6) 0.0395(6) 0.0123(5) 0.0082(5) 0.0134(5) N7 0.0300(5) 0.0242(5) 0.0392(6) 0.0068(4) -0.0002(4) 0.0139(4) C30 0.0219(6) 0.0218(5) 0.0278(6) 0.0040(4) 0.0001(5) 0.0112(5) C31 0.0183(5) 0.0215(6) 0.0262(5) 0.0020(4) 0.0000(4) 0.0087(4) C32 0.0202(5) 0.0177(5) 0.0226(5) 0.0025(4) 0.0000(4) 0.0078(4) C33 0.0192(5) 0.0161(5) 0.0196(5) 0.0006(4) -0.0016(4) 0.0063(4) C34 0.0215(6) 0.0165(5) 0.0210(5) 0.0037(4) -0.0003(4) 0.0067(4) C35 0.0197(5) 0.0175(5) 0.0212(5) 0.0038(4) 0.0009(4) 0.0060(4) _geom_special_details ; All esds (except the esd in the dihedral angle between two l.s. planes) are estimated using the full covariance matrix. The cell esds are taken into account individually in the estimation of esds in distances, angles and torsion angles; correlations between esds in cell parameters are only used when they are defined by crystal symmetry. An approximate (isotropic) treatment of cell esds is used for estimating esds involving l.s. planes. ; loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_distance _geom_bond_site_symmetry_2 _geom_bond_publ_flag N1 C1 1.3380(15) . ? N1 C5 1.3433(15) . ? C1 H1 0.9500 . ? C1 C2 1.3865(16) . ? C2 H2 0.9500 . ? C2 C3 1.3974(15) . ? C3 C4 1.3994(15) . ? C3 C6 1.4632(16) . ? C4 H4 0.9500 . ? C4 C5 1.3823(16) . ? C5 H5 0.9500 . ? C6 H6 0.9500 . ? C6 C7 1.3391(16) . ? C7 H7 0.9500 . ? C7 C8 1.4719(15) . ? C8 C9 1.3862(15) . ? C8 C17 1.4360(15) . ? C9 H9 0.9500 . ? C9 C10 1.4049(16) . ? C10 H10 0.9500 . ? C10 C11 1.3683(16) . ? C11 H11 0.9500 . ? C11 C12 1.4123(15) . ? C12 C13 1.4170(16) . ? C12 C17 1.4315(15) . ? C13 H13 0.9500 . ? C13 C14 1.3697(17) . ? C14 H14 0.9500 . ? C14 C15 1.4111(17) . ? C15 H15 0.9500 . ? C15 C16 1.3701(16) . ? C16 H16 0.9500 . ? C16 C17 1.4224(15) . ? N2 C18 1.1498(16) . ? N3 C19 1.1470(15) . ? N4 C28 1.1496(15) . ? N5 C29 1.1431(15) . ? C18 C20 1.4388(15) . ? C19 C20 1.4354(15) . ? C20 C21 1.3769(15) . ? C21 C22 1.4494(15) . ? C21 C26 1.4477(14) . ? C22 H22 0.9500 . ? C22 C23 1.3499(15) . ? C23 H23 0.9500 . ? C23 C24 1.4499(14) . ? C24 C25 1.4467(14) . ? C24 C27 1.3743(15) . ? C25 H25 0.9500 . ? C25 C26 1.3402(15) . ? C26 H26 0.9500 . ? C27 C28 1.4322(15) . ? C27 C29 1.4389(15) . ? N6 C30 1.1482(16) . ? N7 C31 1.1454(15) . ? C30 C32 1.4342(15) . ? C31 C32 1.4333(15) . ? C32 C33 1.3758(15) . ? C33 C34 1.4483(15) . ? C33 C35 1.4463(14) . ? C34 H34 0.9500 . ? C34 C35 1.3428(15) 2_665 ? C35 H35 0.9500 . ? loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle_publ_flag C1 N1 C5 115.57(10) . . ? N1 C1 H1 117.9 . . ? N1 C1 C2 124.17(11) . . ? C2 C1 H1 117.9 . . ? C1 C2 H2 120.0 . . ? C1 C2 C3 119.91(11) . . ? C3 C2 H2 120.0 . . ? C2 C3 C4 116.21(10) . . ? C2 C3 C6 119.62(10) . . ? C4 C3 C6 124.17(10) . . ? C3 C4 H4 120.3 . . ? C5 C4 C3 119.46(10) . . ? C5 C4 H4 120.3 . . ? N1 C5 C4 124.66(10) . . ? N1 C5 H5 117.7 . . ? C4 C5 H5 117.7 . . ? C3 C6 H6 117.2 . . ? C7 C6 C3 125.51(10) . . ? C7 C6 H6 117.2 . . ? C6 C7 H7 117.0 . . ? C6 C7 C8 125.99(10) . . ? C8 C7 H7 117.0 . . ? C9 C8 C7 120.72(10) . . ? C9 C8 C17 118.71(10) . . ? C17 C8 C7 120.47(9) . . ? C8 C9 H9 119.1 . . ? C8 C9 C10 121.78(10) . . ? C10 C9 H9 119.1 . . ? C9 C10 H10 119.8 . . ? C11 C10 C9 120.35(10) . . ? C11 C10 H10 119.8 . . ? C10 C11 H11 119.8 . . ? C10 C11 C12 120.35(10) . . ? C12 C11 H11 119.8 . . ? C11 C12 C13 120.67(10) . . ? C11 C12 C17 119.88(11) . . ? C13 C12 C17 119.45(10) . . ? C12 C13 H13 119.3 . . ? C14 C13 C12 121.45(11) . . ? C14 C13 H13 119.3 . . ? C13 C14 H14 120.4 . . ? C13 C14 C15 119.20(11) . . ? C15 C14 H14 120.4 . . ? C14 C15 H15 119.5 . . ? C16 C15 C14 121.02(11) . . ? C16 C15 H15 119.5 . . ? C15 C16 H16 119.3 . . ? C15 C16 C17 121.32(10) . . ? C17 C16 H16 119.3 . . ? C12 C17 C8 118.74(10) . . ? C16 C17 C8 123.75(10) . . ? C16 C17 C12 117.51(10) . . ? N2 C18 C20 178.55(12) . . ? N3 C19 C20 176.44(11) . . ? C19 C20 C18 115.22(9) . . ? C21 C20 C18 120.38(10) . . ? C21 C20 C19 124.38(10) . . ? C20 C21 C22 121.88(10) . . ? C20 C21 C26 119.81(10) . . ? C26 C21 C22 118.30(9) . . ? C21 C22 H22 119.8 . . ? C23 C22 C21 120.33(10) . . ? C23 C22 H22 119.8 . . ? C22 C23 H23 119.5 . . ? C22 C23 C24 120.99(10) . . ? C24 C23 H23 119.5 . . ? C25 C24 C23 118.39(9) . . ? C27 C24 C23 121.76(10) . . ? C27 C24 C25 119.85(9) . . ? C24 C25 H25 119.7 . . ? C26 C25 C24 120.56(10) . . ? C26 C25 H25 119.7 . . ? C21 C26 H26 119.3 . . ? C25 C26 C21 121.33(10) . . ? C25 C26 H26 119.3 . . ? C24 C27 C28 123.63(10) . . ? C24 C27 C29 122.57(10) . . ? C28 C27 C29 113.80(9) . . ? N4 C28 C27 175.58(11) . . ? N5 C29 C27 177.29(12) . . ? N6 C30 C32 179.17(12) . . ? N7 C31 C32 178.37(12) . . ? C31 C32 C30 115.29(9) . . ? C33 C32 C30 121.85(10) . . ? C33 C32 C31 122.86(10) . . ? C32 C33 C34 120.77(10) . . ? C32 C33 C35 120.76(10) . . ? C35 C33 C34 118.47(10) . . ? C33 C34 H34 119.9 . . ? C35 C34 C33 120.24(10) 2_665 . ? C35 C34 H34 119.9 2_665 . ? C33 C35 H35 119.4 . . ? C34 C35 C33 121.29(10) 2_665 . ? C34 C35 H35 119.4 2_665 . ? loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion_publ_flag N1 C1 C2 C3 -1.12(19) . . . . ? C1 N1 C5 C4 0.54(17) . . . . ? C1 C2 C3 C4 1.48(17) . . . . ? C1 C2 C3 C6 -178.66(11) . . . . ? C2 C3 C4 C5 -0.91(16) . . . . ? C2 C3 C6 C7 170.55(11) . . . . ? C3 C4 C5 N1 -0.10(18) . . . . ? C3 C6 C7 C8 177.30(10) . . . . ? C4 C3 C6 C7 -9.60(19) . . . . ? C5 N1 C1 C2 0.08(17) . . . . ? C6 C3 C4 C5 179.23(11) . . . . ? C6 C7 C8 C9 8.48(18) . . . . ? C6 C7 C8 C17 -167.77(11) . . . . ? C7 C8 C9 C10 -172.92(10) . . . . ? C7 C8 C17 C12 171.41(10) . . . . ? C7 C8 C17 C16 -8.47(16) . . . . ? C8 C9 C10 C11 0.39(18) . . . . ? C9 C8 C17 C12 -4.92(15) . . . . ? C9 C8 C17 C16 175.21(10) . . . . ? C9 C10 C11 C12 -2.59(17) . . . . ? C10 C11 C12 C13 -178.80(11) . . . . ? C10 C11 C12 C17 0.92(17) . . . . ? C11 C12 C13 C14 177.97(11) . . . . ? C11 C12 C17 C8 2.84(16) . . . . ? C11 C12 C17 C16 -177.28(10) . . . . ? C12 C13 C14 C15 -0.28(17) . . . . ? C13 C12 C17 C8 -177.44(9) . . . . ? C13 C12 C17 C16 2.45(16) . . . . ? C13 C14 C15 C16 1.61(17) . . . . ? C14 C15 C16 C17 -0.84(17) . . . . ? C15 C16 C17 C8 178.69(10) . . . . ? C15 C16 C17 C12 -1.19(16) . . . . ? C17 C8 C9 C10 3.39(16) . . . . ? C17 C12 C13 C14 -1.76(17) . . . . ? C18 C20 C21 C22 -177.19(10) . . . . ? C18 C20 C21 C26 2.03(16) . . . . ? C19 C20 C21 C22 1.39(17) . . . . ? C19 C20 C21 C26 -179.39(10) . . . . ? C20 C21 C22 C23 176.29(10) . . . . ? C20 C21 C26 C25 -176.35(10) . . . . ? C21 C22 C23 C24 0.66(16) . . . . ? C22 C21 C26 C25 2.89(16) . . . . ? C22 C23 C24 C25 1.73(15) . . . . ? C22 C23 C24 C27 -178.23(10) . . . . ? C23 C24 C25 C26 -1.80(15) . . . . ? C23 C24 C27 C28 -1.21(17) . . . . ? C23 C24 C27 C29 179.40(10) . . . . ? C24 C25 C26 C21 -0.53(16) . . . . ? C25 C24 C27 C28 178.83(10) . . . . ? C25 C24 C27 C29 -0.57(17) . . . . ? C26 C21 C22 C23 -2.94(15) . . . . ? C27 C24 C25 C26 178.17(11) . . . . ? C30 C32 C33 C34 177.46(10) . . . . ? C30 C32 C33 C35 -2.14(16) . . . . ? C31 C32 C33 C34 -2.74(17) . . . . ? C31 C32 C33 C35 177.65(10) . . . . ? C32 C33 C34 C35 -178.83(10) . . . 2_665 ? C32 C33 C35 C34 178.82(10) . . . 2_665 ? C34 C33 C35 C34 -0.79(17) . . . 2_665 ? C35 C33 C34 C35 0.78(17) . . . 2_665 ? _shelx_res_file ; TITL CY_B8b in P-1 #2 cy_b8b.res created by SHELXL-2018/3 at 10:31:54 on 28-Jun-2022 REM reset to P-1 #2 CELL 1.54184 9.886245 11.812746 12.310211 93.8271 93.9401 111.868 ZERR 2 0.000359 0.00046 0.000452 0.0031 0.003 0.0035 LATT 1 SFAC C H N UNIT 70 38 14 L.S. 10 PLAN 5 SIZE 0.044 0.186 0.421 TEMP -171 CONF BOND MORE -1 BOND $H fmap 2 acta REM REM REM WGHT 0.065000 0.166600 FVAR 2.90920 N1 3 0.175485 0.281318 0.514085 11.00000 0.02482 0.02425 = 0.02424 0.00434 0.00186 0.00988 C1 1 0.119437 0.367919 0.506504 11.00000 0.02478 0.02672 = 0.02790 0.00493 0.00733 0.01136 AFIX 43 H1 2 0.034055 0.358667 0.541900 11.00000 -1.20000 AFIX 0 C2 1 0.178034 0.470304 0.450280 11.00000 0.02448 0.02417 = 0.02959 0.00482 0.00607 0.01257 AFIX 43 H2 2 0.131912 0.527785 0.446903 11.00000 -1.20000 AFIX 0 C3 1 0.305026 0.488833 0.398585 11.00000 0.01957 0.02251 = 0.02181 0.00171 0.00055 0.00794 C4 1 0.363648 0.398157 0.405512 11.00000 0.02026 0.02375 = 0.02658 0.00242 0.00269 0.00918 AFIX 43 H4 2 0.449089 0.404840 0.371155 11.00000 -1.20000 AFIX 0 C5 1 0.296228 0.298786 0.462749 11.00000 0.02206 0.02197 = 0.02615 0.00224 0.00007 0.00999 AFIX 43 H5 2 0.338279 0.238556 0.466013 11.00000 -1.20000 AFIX 0 C6 1 0.368071 0.598457 0.341441 11.00000 0.02352 0.02289 = 0.02532 0.00379 0.00235 0.01070 AFIX 43 H6 2 0.311646 0.647548 0.331841 11.00000 -1.20000 AFIX 0 C7 1 0.498600 0.635426 0.301532 11.00000 0.02201 0.02003 = 0.02143 0.00179 0.00083 0.00897 AFIX 43 H7 2 0.556571 0.588129 0.314112 11.00000 -1.20000 AFIX 0 C8 1 0.560505 0.742602 0.239969 11.00000 0.02061 0.01776 = 0.02147 0.00017 -0.00072 0.00754 C9 1 0.492451 0.825510 0.230261 11.00000 0.02173 0.02109 = 0.02823 0.00099 0.00195 0.00908 AFIX 43 H9 2 0.411472 0.817679 0.270660 11.00000 -1.20000 AFIX 0 C10 1 0.539992 0.920804 0.162294 11.00000 0.02648 0.01912 = 0.03172 0.00101 -0.00169 0.01271 AFIX 43 H10 2 0.491486 0.976511 0.157705 11.00000 -1.20000 AFIX 0 C11 1 0.655782 0.933808 0.102672 11.00000 0.02776 0.01692 = 0.02556 0.00351 -0.00180 0.00779 AFIX 43 H11 2 0.684685 0.996401 0.054619 11.00000 -1.20000 AFIX 0 C12 1 0.732558 0.854672 0.112187 11.00000 0.02147 0.01662 = 0.02190 0.00085 -0.00112 0.00539 C13 1 0.854303 0.869046 0.052276 11.00000 0.02421 0.02138 = 0.02457 0.00355 0.00179 0.00462 AFIX 43 H13 2 0.882111 0.931018 0.003559 11.00000 -1.20000 AFIX 0 C14 1 0.932771 0.795555 0.063059 11.00000 0.02192 0.02796 = 0.02803 -0.00036 0.00443 0.00785 AFIX 43 H14 2 1.013853 0.806153 0.022041 11.00000 -1.20000 AFIX 0 C15 1 0.891732 0.703911 0.135827 11.00000 0.02316 0.02336 = 0.02746 -0.00016 0.00028 0.01158 AFIX 43 H15 2 0.947368 0.654118 0.144970 11.00000 -1.20000 AFIX 0 C16 1 0.772885 0.685630 0.193499 11.00000 0.02279 0.01830 = 0.02310 0.00156 -0.00039 0.00869 AFIX 43 H16 2 0.746817 0.622579 0.241222 11.00000 -1.20000 AFIX 0 C17 1 0.687758 0.759168 0.183346 11.00000 0.02044 0.01579 = 0.01972 0.00054 -0.00053 0.00584 N2 3 0.362233 0.134059 0.189718 11.00000 0.02791 0.03492 = 0.03429 0.01205 0.01039 0.01679 N3 3 0.160505 -0.181510 0.367847 11.00000 0.02367 0.02699 = 0.03399 0.00775 0.00609 0.01351 N4 3 -0.514954 0.109234 0.459918 11.00000 0.03079 0.03530 = 0.04468 0.01938 0.01612 0.02140 N5 3 -0.282849 0.401125 0.277707 11.00000 0.03604 0.02534 = 0.03545 0.00822 0.00516 0.01657 C18 1 0.264475 0.078170 0.234610 11.00000 0.02307 0.02672 = 0.02294 0.00478 0.00326 0.01439 C19 1 0.148313 -0.096751 0.335185 11.00000 0.01661 0.02606 = 0.02277 0.00213 0.00396 0.00987 C20 1 0.141743 0.011071 0.291724 11.00000 0.01955 0.02153 = 0.01978 0.00220 0.00131 0.00890 C21 1 0.030001 0.052444 0.303711 11.00000 0.01852 0.02018 = 0.01765 0.00091 0.00002 0.00713 C22 1 -0.092003 -0.009728 0.364917 11.00000 0.01964 0.01744 = 0.01982 0.00365 0.00071 0.00723 AFIX 43 H22 2 -0.099194 -0.083821 0.394407 11.00000 -1.20000 AFIX 0 C23 1 -0.195463 0.037119 0.380228 11.00000 0.01871 0.01910 = 0.01881 0.00363 0.00189 0.00656 AFIX 43 H23 2 -0.274325 -0.004066 0.421154 11.00000 -1.20000 AFIX 0 C24 1 -0.188039 0.149346 0.335153 11.00000 0.01861 0.01937 = 0.01778 0.00181 -0.00083 0.00778 C25 1 -0.069118 0.208372 0.270542 11.00000 0.02003 0.02007 = 0.02064 0.00530 0.00219 0.00773 AFIX 43 H25 2 -0.063831 0.280694 0.238521 11.00000 -1.20000 AFIX 0 C26 1 0.033652 0.161889 0.255478 11.00000 0.01890 0.02130 = 0.02101 0.00598 0.00366 0.00719 AFIX 43 H26 2 0.110446 0.201556 0.212279 11.00000 -1.20000 AFIX 0 C27 1 -0.290250 0.200070 0.352404 11.00000 0.02023 0.02074 = 0.02066 0.00416 0.00265 0.00907 C28 1 -0.412852 0.146819 0.413511 11.00000 0.02472 0.02391 = 0.02791 0.00827 0.00458 0.01571 C29 1 -0.283950 0.311962 0.309232 11.00000 0.02143 0.02365 = 0.02477 0.00327 0.00378 0.01163 N6 3 0.062133 0.468792 0.145454 11.00000 0.02631 0.03147 = 0.03953 0.01226 0.00821 0.01342 N7 3 0.258436 0.774667 -0.044901 11.00000 0.02998 0.02421 = 0.03920 0.00682 -0.00025 0.01387 C30 1 0.157145 0.519338 0.096025 11.00000 0.02186 0.02175 = 0.02782 0.00399 0.00012 0.01118 C31 1 0.266243 0.688832 -0.011563 11.00000 0.01828 0.02151 = 0.02624 0.00197 0.00005 0.00873 C32 1 0.274341 0.582194 0.032924 11.00000 0.02024 0.01769 = 0.02262 0.00251 0.00004 0.00780 C33 1 0.386308 0.542240 0.017069 11.00000 0.01919 0.01609 = 0.01961 0.00058 -0.00162 0.00631 C34 1 0.500186 0.604417 -0.050689 11.00000 0.02152 0.01650 = 0.02101 0.00370 -0.00035 0.00666 AFIX 43 H34 2 0.498944 0.674544 -0.083626 11.00000 -1.20000 AFIX 0 C35 1 0.392486 0.436700 0.067122 11.00000 0.01975 0.01754 = 0.02121 0.00382 0.00091 0.00604 AFIX 43 H35 2 0.319180 0.395668 0.112512 11.00000 -1.20000 AFIX 0 HKLF 4 REM CY_B8b in P-1 #2 REM wR2 = 0.1073, GooF = S = 1.031, Restrained GooF = 1.031 for all data REM R1 = 0.0372 for 4451 Fo > 4sig(Fo) and 0.0431 for all 5154 data REM 379 parameters refined using 0 restraints END WGHT 0.0650 0.1666 REM Highest difference peak 0.274, deepest hole -0.195, 1-sigma level 0.043 Q1 1 0.7161 0.8175 0.1472 11.00000 0.05 0.27 Q2 1 0.3842 0.4885 0.0439 11.00000 0.05 0.23 Q3 1 -0.1874 0.0902 0.3552 11.00000 0.05 0.21 Q4 1 -0.1276 0.1776 0.3004 11.00000 0.05 0.20 Q5 1 0.4536 0.5771 -0.0177 11.00000 0.05 0.20 ; _shelx_res_checksum 74300 _olex2_submission_special_instructions 'No special instructions were received' _oxdiff_exptl_absorpt_empirical_details ; Empirical correction (ABSPACK) includes: - Absorption correction using spherical harmonics - Frame scaling ; _oxdiff_exptl_absorpt_empirical_full_max 1.150 _oxdiff_exptl_absorpt_empirical_full_min 0.885 ####################################################################### # # This file contains crystal structure data downloaded from the # Cambridge Structural Database (CSD) hosted by the Cambridge # Crystallographic Data Centre (CCDC). # # Full information about CCDC data access policies and citation # guidelines are available at http://www.ccdc.cam.ac.uk/access/V1 # # Audit and citation data items may have been added by the CCDC. # Please retain this information to preserve the provenance of # this file and to allow appropriate attribution of the data. # ####################################################################### data_Npe-TCNB _database_code_depnum_ccdc_archive 'CCDC 2286628' loop_ _audit_author_name _audit_author_address 'Joseph E. Reynolds III ' ;Sandia National laboratory United States of America ; _audit_update_record ; 2023-08-03 deposited with the CCDC. 2023-09-26 downloaded from the CCDC. ; _audit_creation_date 2022-06-28 _audit_creation_method ; Olex2 1.5 (compiled 2021.12.09 svn.r5202d8cf for OlexSys, GUI svn.r6439) ; _shelx_SHELXL_version_number 2018/3 _chemical_name_common ? _chemical_name_systematic ; ? ; _chemical_formula_moiety 'C10 H2 N4, C17 H13 N' _chemical_formula_sum 'C27 H15 N5' _chemical_formula_weight 409.44 _chemical_melting_point ? _chemical_oxdiff_formula N5C26H15 _chemical_oxdiff_usercomment '1:1 acetonitrile:DMF' loop_ _atom_type_symbol _atom_type_description _atom_type_scat_dispersion_real _atom_type_scat_dispersion_imag _atom_type_scat_source C C 0.0181 0.0091 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' H H 0.0000 0.0000 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' N N 0.0311 0.0180 'International Tables Vol C Tables 4.2.6.8 and 6.1.1.4' _shelx_space_group_comment ; The symmetry employed for this shelxl refinement is uniquely defined by the following loop, which should always be used as a source of symmetry information in preference to the above space-group names. They are only intended as comments. ; _space_group_crystal_system monoclinic _space_group_IT_number 14 _space_group_name_H-M_alt 'P 1 21/c 1' _space_group_name_Hall '-P 2ybc' loop_ _space_group_symop_operation_xyz 'x, y, z' '-x, y+1/2, -z+1/2' '-x, -y, -z' 'x, -y-1/2, z-1/2' _cell_length_a 6.7312(3) _cell_length_b 36.6599(13) _cell_length_c 9.5150(4) _cell_angle_alpha 90 _cell_angle_beta 106.283(4) _cell_angle_gamma 90 _cell_volume 2253.79(17) _cell_formula_units_Z 4 _cell_measurement_reflns_used 2625 _cell_measurement_temperature 99.95(10) _cell_measurement_theta_max 68.1260 _cell_measurement_theta_min 4.7860 _shelx_estimated_absorpt_T_max ? _shelx_estimated_absorpt_T_min ? _exptl_absorpt_coefficient_mu 0.586 _exptl_absorpt_correction_T_max 1.00000 _exptl_absorpt_correction_T_min 0.87727 _exptl_absorpt_correction_type multi-scan _exptl_absorpt_process_details ; CrysAlisPro 1.171.39.46 (Rigaku Oxford Diffraction, 2018) Empirical absorption correction using spherical harmonics, implemented in SCALE3 ABSPACK scaling algorithm. ; _exptl_absorpt_special_details ? _exptl_crystal_colour 'clear yellow' _exptl_crystal_colour_lustre clear _exptl_crystal_colour_modifier . _exptl_crystal_colour_primary yellow _exptl_crystal_density_diffrn 1.207 _exptl_crystal_density_meas ? _exptl_crystal_density_method 'not measured' _exptl_crystal_description plate _exptl_crystal_F_000 848 _exptl_crystal_preparation 'cryoloop with paratone oil' _exptl_crystal_recrystallization_method 'slow evaporation / 1:1 DMF:MeCN' _exptl_crystal_size_max 0.17 _exptl_crystal_size_mid 0.077 _exptl_crystal_size_min 0.037 _exptl_special_details ; ? ; _exptl_transmission_factor_max ? _exptl_transmission_factor_min ? _diffrn_reflns_av_R_equivalents 0.0264 _diffrn_reflns_av_unetI/netI 0.0314 _diffrn_reflns_Laue_measured_fraction_full 0.996 _diffrn_reflns_Laue_measured_fraction_max 0.972 _diffrn_reflns_limit_h_max 6 _diffrn_reflns_limit_h_min -8 _diffrn_reflns_limit_k_max 39 _diffrn_reflns_limit_k_min -44 _diffrn_reflns_limit_l_max 11 _diffrn_reflns_limit_l_min -11 _diffrn_reflns_number 8966 _diffrn_reflns_point_group_measured_fraction_full 0.996 _diffrn_reflns_point_group_measured_fraction_max 0.972 _diffrn_reflns_theta_full 67.684 _diffrn_reflns_theta_max 72.129 _diffrn_reflns_theta_min 4.825 _diffrn_ambient_environment N~2~ _diffrn_ambient_temperature 99.95(10) _diffrn_detector 'CCD plate' _diffrn_detector_area_resol_mean 10.2358 _diffrn_detector_type Atlas _diffrn_measured_fraction_theta_full 0.996 _diffrn_measured_fraction_theta_max 0.972 _diffrn_measurement_details ; List of Runs (angles in degrees, time in seconds): # Type Start End Width t~exp~ \w \q \k \f Frames #-------------------------------------------------------------------------- 1 \w -55.00 32.00 1.00 22.50 -- -42.47 38.00 0.00 87 2 \w -76.00 26.00 1.00 22.50 -- -42.47 19.00 -90.00 102 3 \w 73.00 174.00 1.00 65.00 -- 102.45 61.00 -60.00 101 4 \w 123.00 155.00 1.00 65.00 -- 102.45 125.00 -60.00 32 5 \w 101.00 132.00 1.00 65.00 -- 102.45 -61.00-150.00 31 6 \w 30.00 77.00 1.00 65.00 -- 102.45 -61.00-150.00 47 7 \w 74.00 160.00 1.00 65.00 -- 102.45 61.00 30.00 86 8 \w 112.00 143.00 1.00 65.00 -- 102.45 77.00 -30.00 31 9 \w 98.00 135.00 1.00 65.00 -- 102.45 125.00 -30.00 37 10 \w 138.00 164.00 1.00 65.00 -- 102.45 125.00 -30.00 26 11 \w 132.00 178.00 1.00 65.00 -- 102.45 77.00 120.00 46 ; _diffrn_measurement_device 'four-circle diffractometer' _diffrn_measurement_device_type 'SuperNova, Dual, Cu at home/near, Atlas' _diffrn_measurement_method '\w scans' _diffrn_orient_matrix_type 'CrysAlisPro convention (1999,Acta A55,543-557)' _diffrn_orient_matrix_UB_11 -0.1730409000 _diffrn_orient_matrix_UB_12 0.0287689000 _diffrn_orient_matrix_UB_13 -0.0304468000 _diffrn_orient_matrix_UB_21 0.0994812000 _diffrn_orient_matrix_UB_22 0.0173632000 _diffrn_orient_matrix_UB_23 0.1505777000 _diffrn_orient_matrix_UB_31 0.1297588000 _diffrn_orient_matrix_UB_32 0.0251040000 _diffrn_orient_matrix_UB_33 -0.0690603000 _diffrn_radiation_monochromator mirror _diffrn_radiation_probe x-ray _diffrn_radiation_type 'Cu K\a' _diffrn_radiation_wavelength 1.54184 _diffrn_source 'micro-focus sealed X-ray tube' _diffrn_source_type 'SuperNova (Cu) X-ray Source' _reflns_Friedel_coverage 0.000 _reflns_Friedel_fraction_full . _reflns_Friedel_fraction_max . _reflns_number_gt 3702 _reflns_number_total 4325 _reflns_special_details ; Reflections were merged by SHELXL according to the crystal class for the calculation of statistics and refinement. Structure factors included contributions from the .fab file. _reflns_Friedel_fraction is defined as the number of unique Friedel pairs measured divided by the number that would be possible theoretically, ignoring centric projections and systematic absences. ; _reflns_threshold_expression 'I > 2\s(I)' _computing_cell_refinement 'CrysAlisPro 1.171.39.46 (Rigaku OD, 2018)' _computing_data_collection 'CrysAlisPro 1.171.39.46 (Rigaku OD, 2018)' _computing_data_reduction 'CrysAlisPro 1.171.39.46 (Rigaku OD, 2018)' _computing_molecular_graphics 'Olex2 1.5 (Dolomanov et al., 2009)' _computing_publication_material 'Olex2 1.5 (Dolomanov et al., 2009)' _computing_structure_refinement 'SHELXL 2018/3 (Sheldrick, 2015)' _computing_structure_solution 'SHELXS (Sheldrick, 2008)' _refine_diff_density_max 0.940 _refine_diff_density_min -0.336 _refine_diff_density_rms 0.086 _refine_ls_extinction_coef . _refine_ls_extinction_method none _refine_ls_goodness_of_fit_ref 1.085 _refine_ls_hydrogen_treatment constr _refine_ls_matrix_type full _refine_ls_number_parameters 353 _refine_ls_number_reflns 4325 _refine_ls_number_restraints 102 _refine_ls_R_factor_all 0.1331 _refine_ls_R_factor_gt 0.1237 _refine_ls_restrained_S_all 1.074 _refine_ls_shift/su_max 0.000 _refine_ls_shift/su_mean 0.000 _refine_ls_structure_factor_coef Fsqd _refine_ls_weighting_details 'w=1/[\s^2^(Fo^2^)+(0.1316P)^2^+8.6783P] where P=(Fo^2^+2Fc^2^)/3' _refine_ls_weighting_scheme calc _refine_ls_wR_factor_gt 0.3330 _refine_ls_wR_factor_ref 0.3397 _refine_special_details ? _olex2_refinement_description ; 1. Fixed Uiso At 1.2 times of: All C(H) groups, All C(H,H) groups 2. Uiso/Uaniso restraints and constraints N1 \\sim N1A: within 2A with sigma of 0.01 and sigma for terminal atoms of 0.02 within 2A C3 \\sim C6 \\sim C3A \\sim C6A: within 2A with sigma of 0.01 and sigma for terminal atoms of 0.02 within 2A C1 \\sim C2 \\sim C4 \\sim C5 \\sim C1A \\sim C2A \\sim C4A \\sim C5A: within 2A with sigma of 0.01 and sigma for terminal atoms of 0.02 within 2A 3. Others Sof(H7B)=Sof(N1A)=Sof(C1A)=Sof(H1A)=Sof(C2A)=Sof(H2A)=Sof(C3A)=Sof(C4A)= Sof(H4A)=Sof(C5A)=Sof(H5A)=Sof(C6A)=Sof(H6A)=1-FVAR(1) Sof(H7A)=Sof(N1)=Sof(C1)=Sof(H1)=Sof(C2)=Sof(H2)=Sof(C3)=Sof(C4)=Sof(H4)= Sof(C5)=Sof(H5)=Sof(C6)=Sof(H6)=FVAR(1) 4.a Aromatic/amide H refined with riding coordinates: C22(H22), C27(H27), C7(H7B), C7(H7A), C9(H9), C10(H10), C11(H11), C13(H13), C14(H14), C15(H15), C16(H16), C1(H1), C2(H2), C4(H4), C5(H5), C6(H6), C1A(H1A), C2A(H2A), C4A(H4A), C5A(H5A), C6A(H6A) ; _atom_sites_solution_hydrogens geom _atom_sites_solution_primary direct _atom_sites_solution_secondary ? loop_ _atom_site_label _atom_site_type_symbol _atom_site_fract_x _atom_site_fract_y _atom_site_fract_z _atom_site_U_iso_or_equiv _atom_site_adp_type _atom_site_occupancy _atom_site_site_symmetry_order _atom_site_calc_flag _atom_site_refinement_flags_posn _atom_site_refinement_flags_adp _atom_site_refinement_flags_occupancy _atom_site_disorder_assembly _atom_site_disorder_group N2 N -0.1655(7) 0.38942(11) 0.6917(4) 0.0414(10) Uani 1 1 d . . . . . N3 N -0.1692(5) 0.28007(10) 0.6873(4) 0.0291(8) Uani 1 1 d . . . . . N4 N -0.4799(5) 0.28317(10) -0.0677(4) 0.0277(8) Uani 1 1 d . . . . . N5 N -0.4820(8) 0.39285(11) -0.0541(4) 0.0460(11) Uani 1 1 d . . . . . C18 C -0.2127(7) 0.37335(11) 0.5830(5) 0.0302(9) Uani 1 1 d . . . . . C19 C -0.2154(6) 0.29570(10) 0.5783(4) 0.0212(8) Uani 1 1 d . . . . . C20 C -0.2705(6) 0.35381(11) 0.4466(4) 0.0236(8) Uani 1 1 d . . . . . C21 C -0.2719(5) 0.31581(10) 0.4430(4) 0.0193(8) Uani 1 1 d . . . . . C22 C -0.3270(5) 0.29740(10) 0.3104(4) 0.0194(8) Uani 1 1 d . . . . . H22 H -0.328818 0.272035 0.308761 0.023 Uiso 1 1 calc R U . . . C23 C -0.3793(5) 0.31691(11) 0.1802(4) 0.0207(8) Uani 1 1 d . . . . . C24 C -0.4354(6) 0.29811(11) 0.0428(4) 0.0213(8) Uani 1 1 d . . . . . C25 C -0.4372(7) 0.37595(12) 0.0508(4) 0.0314(10) Uani 1 1 d . . . . . C26 C -0.3787(6) 0.35522(11) 0.1842(4) 0.0233(8) Uani 1 1 d . . . . . C27 C -0.3236(7) 0.37386(11) 0.3164(4) 0.0275(9) Uani 1 1 d . . . . . H27 H -0.322065 0.399228 0.318375 0.033 Uiso 1 1 calc R U . . . C7 C 0.2421(9) 0.40796(14) 0.4804(5) 0.0441(12) Uani 1 1 d . . . . . H7B H 0.246187 0.422521 0.401188 0.053 Uiso 0.386(8) 1 calc R U P A 2 H7A H 0.169668 0.422119 0.401523 0.053 Uiso 0.614(8) 1 calc R U P A 1 C8 C 0.2322(6) 0.36895(12) 0.4587(4) 0.0281(9) Uani 1 1 d . . . . . C9 C 0.2838(6) 0.34596(14) 0.5803(5) 0.0335(10) Uani 1 1 d . . . . . H9 H 0.323030 0.356064 0.673640 0.040 Uiso 1 1 calc R U . . . C10 C 0.2779(6) 0.30816(13) 0.5647(5) 0.0313(10) Uani 1 1 d . . . . . H10 H 0.313504 0.293450 0.647685 0.038 Uiso 1 1 calc R U . . . C11 C 0.2208(6) 0.29253(12) 0.4300(5) 0.0285(9) Uani 1 1 d . . . . . H11 H 0.215370 0.267254 0.421307 0.034 Uiso 1 1 calc R U . . . C12 C 0.1697(6) 0.31445(11) 0.3034(4) 0.0241(8) Uani 1 1 d . . . . . C13 C 0.1117(6) 0.29794(13) 0.1631(5) 0.0315(10) Uani 1 1 d . . . . . H13 H 0.108054 0.272644 0.155652 0.038 Uiso 1 1 calc R U . . . C14 C 0.0613(7) 0.31844(15) 0.0394(5) 0.0371(11) Uani 1 1 d . . . . . H14 H 0.023848 0.307224 -0.051907 0.045 Uiso 1 1 calc R U . . . C15 C 0.0658(7) 0.35632(15) 0.0497(5) 0.0372(11) Uani 1 1 d . . . . . H15 H 0.031103 0.370177 -0.035600 0.045 Uiso 1 1 calc R U . . . C16 C 0.1207(7) 0.37378(13) 0.1836(4) 0.0316(10) Uani 1 1 d . . . . . H16 H 0.122149 0.399125 0.187545 0.038 Uiso 1 1 calc R U . . . C17 C 0.1750(6) 0.35323(12) 0.3153(4) 0.0247(9) Uani 1 1 d . . . . . N1 N 0.369(2) 0.5411(3) 0.6736(13) 0.073(3) Uani 0.614(8) 1 d . U P A 1 C1 C 0.455(3) 0.5176(3) 0.7748(14) 0.090(4) Uani 0.614(8) 1 d . U P A 1 H1 H 0.525760 0.526408 0.866838 0.108 Uiso 0.614(8) 1 calc R U P A 1 C2 C 0.446(3) 0.4801(3) 0.7532(13) 0.089(4) Uani 0.614(8) 1 d . U P A 1 H2 H 0.507311 0.464851 0.831509 0.107 Uiso 0.614(8) 1 calc R U P A 1 C3 C 0.3468(19) 0.4644(3) 0.6169(11) 0.047(2) Uani 0.614(8) 1 d . U P A 1 C4 C 0.235(4) 0.4911(8) 0.519(4) 0.069(4) Uani 0.614(8) 1 d . U P A 1 H4 H 0.154982 0.483965 0.426876 0.083 Uiso 0.614(8) 1 calc R U P A 1 C5 C 0.243(3) 0.5265(5) 0.556(2) 0.068(4) Uani 0.614(8) 1 d . U P A 1 H5 H 0.150416 0.542043 0.493069 0.082 Uiso 0.614(8) 1 calc R U P A 1 C6 C 0.3409(19) 0.4254(3) 0.5976(12) 0.050(2) Uani 0.614(8) 1 d . U P A 1 H6 H 0.414821 0.411488 0.676654 0.059 Uiso 0.614(8) 1 calc R U P A 1 N1A N 0.235(3) 0.5407(4) 0.692(2) 0.074(4) Uani 0.386(8) 1 d . U P A 2 C1A C 0.217(4) 0.5150(4) 0.788(2) 0.090(4) Uani 0.386(8) 1 d . U P A 2 H1A H 0.189547 0.522230 0.874810 0.108 Uiso 0.386(8) 1 calc R U P A 2 C2A C 0.236(4) 0.4779(5) 0.763(2) 0.088(4) Uani 0.386(8) 1 d . U P A 2 H2A H 0.242069 0.461730 0.838820 0.106 Uiso 0.386(8) 1 calc R U P A 2 C3A C 0.248(3) 0.4644(4) 0.6358(17) 0.044(3) Uani 0.386(8) 1 d . U P A 2 C4A C 0.293(6) 0.4887(14) 0.516(6) 0.069(5) Uani 0.386(8) 1 d . U P A 2 H4A H 0.302441 0.478378 0.428504 0.083 Uiso 0.386(8) 1 calc R U P A 2 C5A C 0.318(5) 0.5252(9) 0.538(4) 0.072(5) Uani 0.386(8) 1 d . U P A 2 H5A H 0.372856 0.540470 0.480246 0.087 Uiso 0.386(8) 1 calc R U P A 2 C6A C 0.246(3) 0.4249(5) 0.6080(19) 0.043(3) Uani 0.386(8) 1 d . U P A 2 H6A H 0.247707 0.409861 0.686882 0.051 Uiso 0.386(8) 1 calc R U P A 2 loop_ _atom_site_aniso_label _atom_site_aniso_U_11 _atom_site_aniso_U_22 _atom_site_aniso_U_33 _atom_site_aniso_U_23 _atom_site_aniso_U_13 _atom_site_aniso_U_12 N2 0.057(3) 0.035(2) 0.028(2) -0.0068(16) 0.0041(18) 0.0042(18) N3 0.0319(19) 0.0301(19) 0.0223(17) 0.0009(14) 0.0028(14) 0.0005(14) N4 0.0285(17) 0.0341(19) 0.0206(17) -0.0014(14) 0.0070(13) -0.0006(14) N5 0.069(3) 0.038(2) 0.028(2) 0.0092(17) 0.0075(19) 0.008(2) C18 0.039(2) 0.024(2) 0.024(2) 0.0019(17) 0.0048(17) 0.0030(17) C19 0.0217(18) 0.0221(18) 0.0207(19) -0.0002(15) 0.0075(14) -0.0009(15) C20 0.026(2) 0.027(2) 0.0170(18) -0.0015(15) 0.0044(15) 0.0006(15) C21 0.0140(16) 0.0260(19) 0.0180(18) 0.0000(14) 0.0046(13) -0.0001(14) C22 0.0186(17) 0.0199(18) 0.0204(18) -0.0008(14) 0.0066(14) -0.0012(14) C23 0.0161(17) 0.027(2) 0.0185(18) -0.0014(15) 0.0041(14) 0.0008(14) C24 0.0169(17) 0.0282(19) 0.0186(18) 0.0010(15) 0.0049(14) -0.0001(14) C25 0.046(3) 0.026(2) 0.021(2) 0.0002(17) 0.0083(18) 0.0032(18) C26 0.026(2) 0.027(2) 0.0163(18) 0.0015(15) 0.0043(15) 0.0029(15) C27 0.039(2) 0.0219(19) 0.0205(19) 0.0024(15) 0.0063(17) 0.0022(17) C7 0.061(3) 0.035(3) 0.034(2) 0.003(2) 0.009(2) 0.001(2) C8 0.025(2) 0.033(2) 0.026(2) -0.0039(17) 0.0062(16) -0.0014(16) C9 0.023(2) 0.057(3) 0.0190(19) -0.0045(18) 0.0042(16) -0.0016(19) C10 0.021(2) 0.045(3) 0.027(2) 0.0103(18) 0.0053(16) -0.0003(18) C11 0.0194(19) 0.032(2) 0.036(2) 0.0069(17) 0.0104(16) 0.0037(16) C12 0.0155(17) 0.032(2) 0.026(2) 0.0019(16) 0.0075(15) -0.0018(15) C13 0.0196(19) 0.039(2) 0.037(2) -0.0114(19) 0.0103(17) -0.0058(17) C14 0.023(2) 0.064(3) 0.024(2) -0.011(2) 0.0069(17) -0.008(2) C15 0.029(2) 0.064(3) 0.019(2) 0.005(2) 0.0067(17) 0.002(2) C16 0.037(2) 0.036(2) 0.022(2) 0.0044(17) 0.0083(17) 0.0016(18) C17 0.0226(19) 0.033(2) 0.0169(18) -0.0011(15) 0.0026(15) 0.0010(16) N1 0.098(8) 0.034(4) 0.083(6) -0.003(4) 0.017(6) -0.002(6) C1 0.162(10) 0.041(5) 0.059(5) 0.001(4) 0.016(6) -0.007(6) C2 0.163(10) 0.037(4) 0.057(5) -0.005(4) 0.011(6) -0.009(6) C3 0.065(6) 0.041(4) 0.038(4) -0.001(3) 0.018(4) 0.009(5) C4 0.086(13) 0.039(5) 0.078(5) 0.003(4) 0.017(8) 0.012(8) C5 0.087(12) 0.042(4) 0.076(6) -0.002(4) 0.023(7) 0.016(7) C6 0.065(6) 0.041(4) 0.040(4) 0.001(3) 0.011(5) 0.004(5) N1A 0.089(10) 0.039(6) 0.080(8) 0.005(6) -0.001(9) -0.008(8) C1A 0.162(11) 0.033(6) 0.057(7) -0.006(5) 0.004(8) 0.001(7) C2A 0.160(11) 0.036(6) 0.052(6) -0.012(5) 0.003(8) 0.005(7) C3A 0.058(7) 0.038(5) 0.040(5) 0.003(4) 0.022(5) 0.005(6) C4A 0.091(14) 0.038(6) 0.078(6) -0.001(5) 0.020(9) 0.014(9) C5A 0.091(14) 0.041(6) 0.080(7) -0.003(6) 0.017(9) 0.012(9) C6A 0.059(7) 0.038(5) 0.034(5) -0.001(4) 0.017(6) 0.005(6) _geom_special_details ; All esds (except the esd in the dihedral angle between two l.s. planes) are estimated using the full covariance matrix. The cell esds are taken into account individually in the estimation of esds in distances, angles and torsion angles; correlations between esds in cell parameters are only used when they are defined by crystal symmetry. An approximate (isotropic) treatment of cell esds is used for estimating esds involving l.s. planes. ; loop_ _geom_bond_atom_site_label_1 _geom_bond_atom_site_label_2 _geom_bond_distance _geom_bond_site_symmetry_2 _geom_bond_publ_flag N2 C18 1.155(6) . ? N3 C19 1.149(5) . ? N4 C24 1.148(5) . ? N5 C25 1.141(6) . ? C18 C20 1.437(5) . ? C19 C21 1.439(5) . ? C20 C21 1.393(5) . ? C20 C27 1.398(5) . ? C21 C22 1.387(5) . ? C22 H22 0.9300 . ? C22 C23 1.388(5) . ? C23 C24 1.432(5) . ? C23 C26 1.405(5) . ? C25 C26 1.437(5) . ? C26 C27 1.388(5) . ? C27 H27 0.9300 . ? C7 H7B 0.9300 . ? C7 H7A 0.9300 . ? C7 C8 1.444(6) . ? C7 C6 1.296(12) . ? C7 C6A 1.358(17) . ? C8 C9 1.394(6) . ? C8 C17 1.431(5) . ? C9 H9 0.9300 . ? C9 C10 1.393(7) . ? C10 H10 0.9300 . ? C10 C11 1.358(6) . ? C11 H11 0.9300 . ? C11 C12 1.408(6) . ? C12 C13 1.417(6) . ? C12 C17 1.426(6) . ? C13 H13 0.9300 . ? C13 C14 1.357(7) . ? C14 H14 0.9300 . ? C14 C15 1.392(7) . ? C15 H15 0.9300 . ? C15 C16 1.381(6) . ? C16 H16 0.9300 . ? C16 C17 1.419(5) . ? N1 C1 1.300(16) . ? N1 C5 1.31(2) . ? C1 H1 0.9300 . ? C1 C2 1.390(15) . ? C2 H2 0.9300 . ? C2 C3 1.404(15) . ? C3 C4 1.41(3) . ? C3 C6 1.440(14) . ? C4 H4 0.9300 . ? C4 C5 1.34(3) . ? C5 H5 0.9300 . ? C6 H6 0.9300 . ? N1A C1A 1.34(3) . ? N1A C5A 1.80(4) . ? C1A H1A 0.9300 . ? C1A C2A 1.40(2) . ? C2A H2A 0.9300 . ? C2A C3A 1.33(2) . ? C3A C4A 1.55(6) . ? C3A C6A 1.47(2) . ? C4A H4A 0.9300 . ? C4A C5A 1.36(4) . ? C5A H5A 0.9300 . ? C6A H6A 0.9300 . ? loop_ _geom_angle_atom_site_label_1 _geom_angle_atom_site_label_2 _geom_angle_atom_site_label_3 _geom_angle _geom_angle_site_symmetry_1 _geom_angle_site_symmetry_3 _geom_angle_publ_flag N2 C18 C20 179.1(5) . . ? N3 C19 C21 179.0(4) . . ? C21 C20 C18 121.2(3) . . ? C21 C20 C27 120.4(3) . . ? C27 C20 C18 118.4(4) . . ? C20 C21 C19 119.5(3) . . ? C22 C21 C19 120.0(3) . . ? C22 C21 C20 120.5(3) . . ? C21 C22 H22 120.1 . . ? C21 C22 C23 119.8(3) . . ? C23 C22 H22 120.1 . . ? C22 C23 C24 120.2(3) . . ? C22 C23 C26 119.6(3) . . ? C26 C23 C24 120.2(3) . . ? N4 C24 C23 179.7(5) . . ? N5 C25 C26 179.0(5) . . ? C23 C26 C25 120.5(3) . . ? C27 C26 C23 121.0(3) . . ? C27 C26 C25 118.5(4) . . ? C20 C27 H27 120.6 . . ? C26 C27 C20 118.8(4) . . ? C26 C27 H27 120.6 . . ? C8 C7 H7B 117.6 . . ? C8 C7 H7A 116.4 . . ? C6 C7 H7A 116.4 . . ? C6 C7 C8 127.2(7) . . ? C6A C7 H7B 117.6 . . ? C6A C7 C8 124.8(9) . . ? C9 C8 C7 119.3(4) . . ? C9 C8 C17 119.0(4) . . ? C17 C8 C7 121.6(4) . . ? C8 C9 H9 119.3 . . ? C10 C9 C8 121.4(4) . . ? C10 C9 H9 119.3 . . ? C9 C10 H10 119.6 . . ? C11 C10 C9 120.8(4) . . ? C11 C10 H10 119.6 . . ? C10 C11 H11 119.9 . . ? C10 C11 C12 120.2(4) . . ? C12 C11 H11 119.9 . . ? C11 C12 C13 119.9(4) . . ? C11 C12 C17 120.4(4) . . ? C13 C12 C17 119.7(4) . . ? C12 C13 H13 119.5 . . ? C14 C13 C12 121.1(4) . . ? C14 C13 H13 119.5 . . ? C13 C14 H14 120.1 . . ? C13 C14 C15 119.8(4) . . ? C15 C14 H14 120.1 . . ? C14 C15 H15 119.3 . . ? C16 C15 C14 121.5(4) . . ? C16 C15 H15 119.3 . . ? C15 C16 H16 119.8 . . ? C15 C16 C17 120.3(4) . . ? C17 C16 H16 119.8 . . ? C12 C17 C8 118.1(4) . . ? C16 C17 C8 124.2(4) . . ? C16 C17 C12 117.7(4) . . ? C1 N1 C5 113.9(12) . . ? N1 C1 H1 118.2 . . ? N1 C1 C2 123.7(12) . . ? C2 C1 H1 118.2 . . ? C1 C2 H2 119.0 . . ? C1 C2 C3 122.1(11) . . ? C3 C2 H2 119.0 . . ? C2 C3 C4 110.6(17) . . ? C2 C3 C6 120.8(9) . . ? C4 C3 C6 127.8(17) . . ? C3 C4 H4 119.3 . . ? C5 C4 C3 121(2) . . ? C5 C4 H4 119.3 . . ? N1 C5 C4 125.9(16) . . ? N1 C5 H5 117.0 . . ? C4 C5 H5 117.0 . . ? C7 C6 C3 126.1(9) . . ? C7 C6 H6 116.9 . . ? C3 C6 H6 116.9 . . ? C1A N1A C5A 116.3(18) . . ? N1A C1A H1A 118.9 . . ? N1A C1A C2A 122(2) . . ? C2A C1A H1A 118.9 . . ? C1A C2A H2A 118.1 . . ? C3A C2A C1A 123.8(19) . . ? C3A C2A H2A 118.1 . . ? C2A C3A C4A 122(2) . . ? C2A C3A C6A 122.2(15) . . ? C6A C3A C4A 115(2) . . ? C3A C4A H4A 120.2 . . ? C5A C4A C3A 120(4) . . ? C5A C4A H4A 120.2 . . ? N1A C5A H5A 123.7 . . ? C4A C5A N1A 113(3) . . ? C4A C5A H5A 123.7 . . ? C7 C6A C3A 127.6(14) . . ? C7 C6A H6A 116.2 . . ? C3A C6A H6A 116.2 . . ? loop_ _geom_torsion_atom_site_label_1 _geom_torsion_atom_site_label_2 _geom_torsion_atom_site_label_3 _geom_torsion_atom_site_label_4 _geom_torsion _geom_torsion_site_symmetry_1 _geom_torsion_site_symmetry_2 _geom_torsion_site_symmetry_3 _geom_torsion_site_symmetry_4 _geom_torsion_publ_flag C18 C20 C21 C19 0.3(6) . . . . ? C18 C20 C21 C22 -179.6(4) . . . . ? C18 C20 C27 C26 179.7(4) . . . . ? C19 C21 C22 C23 -179.3(3) . . . . ? C20 C21 C22 C23 0.6(5) . . . . ? C21 C20 C27 C26 0.4(6) . . . . ? C21 C22 C23 C24 179.7(3) . . . . ? C21 C22 C23 C26 -0.9(5) . . . . ? C22 C23 C26 C25 -178.5(4) . . . . ? C22 C23 C26 C27 0.9(6) . . . . ? C23 C26 C27 C20 -0.7(6) . . . . ? C24 C23 C26 C25 1.0(6) . . . . ? C24 C23 C26 C27 -179.6(4) . . . . ? C25 C26 C27 C20 178.7(4) . . . . ? C27 C20 C21 C19 179.6(4) . . . . ? C27 C20 C21 C22 -0.3(6) . . . . ? C7 C8 C9 C10 -179.6(4) . . . . ? C7 C8 C17 C12 179.8(4) . . . . ? C7 C8 C17 C16 -1.0(7) . . . . ? C8 C7 C6 C3 -179.4(9) . . . . ? C8 C7 C6A C3A -177.4(13) . . . . ? C8 C9 C10 C11 -0.2(6) . . . . ? C9 C8 C17 C12 1.2(6) . . . . ? C9 C8 C17 C16 -179.6(4) . . . . ? C9 C10 C11 C12 1.0(6) . . . . ? C10 C11 C12 C13 179.6(4) . . . . ? C10 C11 C12 C17 -0.8(6) . . . . ? C11 C12 C13 C14 179.8(4) . . . . ? C11 C12 C17 C8 -0.4(6) . . . . ? C11 C12 C17 C16 -179.6(4) . . . . ? C12 C13 C14 C15 -0.2(6) . . . . ? C13 C12 C17 C8 179.3(4) . . . . ? C13 C12 C17 C16 0.0(6) . . . . ? C13 C14 C15 C16 0.0(7) . . . . ? C14 C15 C16 C17 0.2(7) . . . . ? C15 C16 C17 C8 -179.5(4) . . . . ? C15 C16 C17 C12 -0.2(6) . . . . ? C17 C8 C9 C10 -0.9(6) . . . . ? C17 C12 C13 C14 0.1(6) . . . . ? N1 C1 C2 C3 2(3) . . . . ? C1 N1 C5 C4 -17(2) . . . . ? C1 C2 C3 C4 -9(2) . . . . ? C1 C2 C3 C6 179.7(15) . . . . ? C2 C3 C4 C5 4(3) . . . . ? C2 C3 C6 C7 174.8(13) . . . . ? C3 C4 C5 N1 9(3) . . . . ? C4 C3 C6 C7 6(2) . . . . ? C5 N1 C1 C2 11(3) . . . . ? C6 C7 C8 C9 18.3(10) . . . . ? C6 C7 C8 C17 -160.2(8) . . . . ? C6 C3 C4 C5 174.4(14) . . . . ? N1A C1A C2A C3A -9(4) . . . . ? C1A N1A C5A C4A 18(3) . . . . ? C1A C2A C3A C4A 15(4) . . . . ? C1A C2A C3A C6A -173(2) . . . . ? C2A C3A C4A C5A -1(4) . . . . ? C2A C3A C6A C7 175(2) . . . . ? C3A C4A C5A N1A -14(3) . . . . ? C4A C3A C6A C7 -13(3) . . . . ? C5A N1A C1A C2A -7(3) . . . . ? C6A C7 C8 C9 -17.9(12) . . . . ? C6A C7 C8 C17 163.5(10) . . . . ? C6A C3A C4A C5A -173(2) . . . . ? _smtbx_masks_special_details ? loop_ _smtbx_masks_void_nr _smtbx_masks_void_average_x _smtbx_masks_void_average_y _smtbx_masks_void_average_z _smtbx_masks_void_volume _smtbx_masks_void_count_electrons _smtbx_masks_void_content 1 0.000 0.000 0.500 62.2 27.4 ? 2 0.000 0.500 1.000 62.2 27.4 ? _smtbx_masks_void_probe_radius 1.2 _smtbx_masks_void_truncation_radius 1.2 _shelx_res_file ; TITL cy_d1_a.res in P2(1)/c cy_d1.res created by SHELXL-2018/3 at 10:51:45 on 28-Jun-2022 REM Old TITL CY_D1 in P21/m #11 REM SHELXT solution in P2(1)/c: R1 0.266, Rweak 0.039, Alpha 0.147 REM 4.369 for 89 systematic absences, Orientation as input REM Formula found by SHELXT: C23 N7 CELL 1.54184 6.7312 36.6599 9.515 90 106.283 90 ZERR 4 0.0003 0.0013 0.0004 0 0.004 0 LATT 1 SYMM -X,0.5+Y,0.5-Z SFAC C H N UNIT 108 60 20 SIMU 0.01 0.02 2 N1 N1a SIMU 0.01 0.02 2 C3 C6 C3a C6a SIMU 0.01 0.02 2 C1 C2 C4 C5 C1a C2a C4a C5a L.S. 10 PLAN 5 CONF BOND list 4 MORE -1 BOND $H ABIN fmap 2 acta OMIT -1 1 2 OMIT 0 1 8 OMIT -2 3 2 OMIT 0 1 1 REM REM REM WGHT 0.131600 8.678301 FVAR 0.34192 0.61367 N2 3 -0.165539 0.389417 0.691749 11.00000 0.05662 0.03518 = 0.02778 -0.00675 0.00414 0.00415 N3 3 -0.169231 0.280072 0.687315 11.00000 0.03192 0.03007 = 0.02235 0.00085 0.00277 0.00051 N4 3 -0.479866 0.283169 -0.067667 11.00000 0.02849 0.03408 = 0.02056 -0.00140 0.00700 -0.00065 N5 3 -0.482019 0.392848 -0.054127 11.00000 0.06872 0.03763 = 0.02808 0.00918 0.00749 0.00826 C18 1 -0.212740 0.373346 0.583041 11.00000 0.03926 0.02441 = 0.02437 0.00192 0.00483 0.00301 C19 1 -0.215434 0.295698 0.578283 11.00000 0.02174 0.02209 = 0.02075 -0.00019 0.00751 -0.00085 C20 1 -0.270526 0.353812 0.446632 11.00000 0.02572 0.02703 = 0.01696 -0.00148 0.00440 0.00061 C21 1 -0.271906 0.315813 0.443048 11.00000 0.01404 0.02599 = 0.01803 0.00002 0.00461 -0.00010 C22 1 -0.326962 0.297399 0.310437 11.00000 0.01862 0.01994 = 0.02037 -0.00077 0.00664 -0.00120 AFIX 43 H22 2 -0.328818 0.272035 0.308761 11.00000 -1.20000 AFIX 0 C23 1 -0.379284 0.316911 0.180232 11.00000 0.01613 0.02714 = 0.01845 -0.00142 0.00415 0.00077 C24 1 -0.435375 0.298112 0.042804 11.00000 0.01695 0.02820 = 0.01865 0.00104 0.00492 -0.00005 C25 1 -0.437209 0.375949 0.050751 11.00000 0.04611 0.02647 = 0.02082 0.00017 0.00826 0.00324 C26 1 -0.378675 0.355217 0.184168 11.00000 0.02592 0.02652 = 0.01634 0.00153 0.00429 0.00287 C27 1 -0.323616 0.373865 0.316414 11.00000 0.03877 0.02192 = 0.02050 0.00237 0.00631 0.00221 AFIX 43 H27 2 -0.322065 0.399228 0.318375 11.00000 -1.20000 AFIX 0 C7 1 0.242118 0.407963 0.480376 11.00000 0.06056 0.03511 = 0.03405 0.00281 0.00892 0.00137 PART 2 AFIX 43 H7B 2 0.246187 0.422521 0.401188 -21.00000 -1.20000 AFIX 43 PART 1 H7A 2 0.169668 0.422119 0.401523 21.00000 -1.20000 AFIX 0 PART 0 C8 1 0.232189 0.368954 0.458733 11.00000 0.02549 0.03259 = 0.02559 -0.00395 0.00618 -0.00143 C9 1 0.283818 0.345958 0.580258 11.00000 0.02333 0.05711 = 0.01900 -0.00454 0.00417 -0.00158 AFIX 43 H9 2 0.323030 0.356064 0.673640 11.00000 -1.20000 AFIX 0 C10 1 0.277903 0.308158 0.564745 11.00000 0.02128 0.04460 = 0.02720 0.01028 0.00533 -0.00030 AFIX 43 H10 2 0.313504 0.293450 0.647685 11.00000 -1.20000 AFIX 0 C11 1 0.220792 0.292527 0.430007 11.00000 0.01940 0.03172 = 0.03602 0.00694 0.01045 0.00373 AFIX 43 H11 2 0.215370 0.267254 0.421307 11.00000 -1.20000 AFIX 0 C12 1 0.169729 0.314447 0.303360 11.00000 0.01554 0.03209 = 0.02568 0.00185 0.00748 -0.00179 C13 1 0.111676 0.297944 0.163073 11.00000 0.01955 0.03937 = 0.03700 -0.01142 0.01026 -0.00584 AFIX 43 H13 2 0.108054 0.272644 0.155652 11.00000 -1.20000 AFIX 0 C14 1 0.061294 0.318444 0.039413 11.00000 0.02335 0.06371 = 0.02432 -0.01115 0.00688 -0.00850 AFIX 43 H14 2 0.023848 0.307224 -0.051907 11.00000 -1.20000 AFIX 0 C15 1 0.065834 0.356315 0.049677 11.00000 0.02870 0.06420 = 0.01884 0.00481 0.00674 0.00226 AFIX 43 H15 2 0.031103 0.370177 -0.035600 11.00000 -1.20000 AFIX 0 C16 1 0.120739 0.373776 0.183608 11.00000 0.03721 0.03572 = 0.02200 0.00437 0.00833 0.00161 AFIX 43 H16 2 0.122149 0.399125 0.187545 11.00000 -1.20000 AFIX 0 C17 1 0.175031 0.353234 0.315292 11.00000 0.02259 0.03288 = 0.01695 -0.00109 0.00257 0.00097 PART 1 N1 3 0.369018 0.541105 0.673621 21.00000 0.09797 0.03362 = 0.08306 -0.00324 0.01707 -0.00179 C1 1 0.454610 0.517611 0.774815 21.00000 0.16180 0.04120 = 0.05851 0.00058 0.01580 -0.00743 AFIX 43 H1 2 0.525760 0.526408 0.866838 21.00000 -1.20000 AFIX 0 C2 1 0.445764 0.480068 0.753203 21.00000 0.16251 0.03650 = 0.05703 -0.00488 0.01136 -0.00913 AFIX 43 H2 2 0.507311 0.464851 0.831509 21.00000 -1.20000 AFIX 0 C3 1 0.346840 0.464410 0.616883 21.00000 0.06478 0.04061 = 0.03846 -0.00073 0.01788 0.00882 C4 1 0.235411 0.491083 0.519106 21.00000 0.08638 0.03919 = 0.07822 0.00343 0.01660 0.01238 AFIX 43 H4 2 0.154982 0.483965 0.426876 21.00000 -1.20000 AFIX 0 C5 1 0.242911 0.526467 0.556215 21.00000 0.08718 0.04175 = 0.07644 -0.00158 0.02310 0.01633 AFIX 43 H5 2 0.150416 0.542043 0.493069 21.00000 -1.20000 AFIX 0 C6 1 0.340890 0.425436 0.597610 21.00000 0.06540 0.04107 = 0.04016 0.00116 0.01144 0.00402 AFIX 43 H6 2 0.414821 0.411488 0.676654 21.00000 -1.20000 AFIX 0 PART 2 N1A 3 0.235241 0.540664 0.692339 -21.00000 0.08895 0.03934 = 0.08001 0.00468 -0.00102 -0.00833 C1A 1 0.216592 0.515041 0.788257 -21.00000 0.16230 0.03336 = 0.05688 -0.00635 0.00373 0.00118 AFIX 43 H1A 2 0.189547 0.522230 0.874810 -21.00000 -1.20000 AFIX 0 C2A 1 0.236412 0.477926 0.762567 -21.00000 0.16039 0.03625 = 0.05194 -0.01242 0.00322 0.00465 AFIX 43 H2A 2 0.242069 0.461730 0.838820 -21.00000 -1.20000 AFIX 0 C3A 1 0.247642 0.464413 0.635846 -21.00000 0.05806 0.03786 = 0.03998 0.00302 0.02224 0.00476 C4A 1 0.292835 0.488692 0.515658 -21.00000 0.09052 0.03802 = 0.07771 -0.00143 0.02034 0.01437 AFIX 43 H4A 2 0.302441 0.478378 0.428504 -21.00000 -1.20000 AFIX 0 C5A 1 0.318426 0.525163 0.538070 -21.00000 0.09102 0.04137 = 0.08027 -0.00315 0.01736 0.01156 AFIX 43 H5A 2 0.372856 0.540470 0.480246 -21.00000 -1.20000 AFIX 0 C6A 1 0.245949 0.424948 0.607965 -21.00000 0.05908 0.03766 = 0.03395 -0.00054 0.01716 0.00539 AFIX 43 H6A 2 0.247707 0.409861 0.686882 -21.00000 -1.20000 AFIX 0 HKLF 4 REM cy_d1_a.res in P2(1)/c REM wR2 = 0.3397, GooF = S = 1.085, Restrained GooF = 1.074 for all data REM R1 = 0.1237 for 3702 Fo > 4sig(Fo) and 0.1331 for all 4325 data REM 353 parameters refined using 102 restraints END WGHT 0.1316 8.6800 REM Highest difference peak 0.940, deepest hole -0.336, 1-sigma level 0.086 Q1 1 0.1043 0.4136 0.1516 11.00000 0.05 0.94 Q2 1 -0.0457 0.5342 0.8163 11.00000 0.05 0.65 Q3 1 0.1107 0.5253 0.9387 11.00000 0.05 0.63 Q4 1 0.6606 0.5203 0.8811 11.00000 0.05 0.60 Q5 1 0.0384 0.5126 0.8568 11.00000 0.05 0.54 ; _shelx_res_checksum 25644 _shelx_fab_file ; -8 0 2 -1.4944 -0.0036 -8 0 4 -2.4617 -0.0057 -8 1 2 -0.0709 -0.0050 -8 1 3 2.2093 0.0041 -8 1 4 -0.5255 -0.0189 -8 2 2 -1.1948 -0.0039 -8 2 3 0.5958 0.0110 -8 2 4 -2.0881 -0.0058 -8 3 2 -0.1689 -0.0008 -8 3 3 1.5014 0.0036 -8 3 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0.0021 -1 33 4 -0.0791 -0.0009 -1 33 5 0.4965 0.0002 -1 33 6 0.9002 -0.0027 -1 33 7 -0.4249 -0.0026 -1 34 1 -0.5002 0.0012 -1 34 2 -0.3711 -0.0012 -1 34 3 0.3670 0.0014 -1 34 4 -0.7119 -0.0012 -1 34 5 -0.6349 0.0019 -1 34 6 0.2402 0.0027 -1 34 7 -0.7284 0.0012 -1 35 1 0.0665 -0.0003 -1 35 2 -0.1020 -0.0017 -1 35 3 0.4817 0.0009 -1 35 4 0.0839 -0.0015 -1 35 5 -0.0022 -0.0015 -1 35 6 1.0306 -0.0019 -1 35 7 -0.5047 -0.0032 -1 36 1 -0.2974 0.0012 -1 36 2 -0.2348 0.0008 -1 36 3 0.1990 0.0013 -1 36 4 0.0663 0.0007 -1 36 5 -0.7669 0.0021 -1 36 6 0.4365 0.0035 -1 37 1 0.1965 -0.0021 -1 37 2 -0.1059 -0.0009 -1 37 3 -0.2722 -0.0009 -1 37 4 0.2487 -0.0014 -1 37 5 -0.4904 -0.0026 -1 37 6 0.9657 -0.0009 -1 38 1 -0.0716 0.0007 -1 38 2 0.2303 0.0017 -1 38 3 0.0997 0.0004 -1 38 4 0.7704 0.0017 -1 38 5 -0.7114 0.0018 -1 38 6 0.4885 0.0020 -1 39 1 -0.0525 -0.0017 -1 39 2 -0.2051 0.0004 -1 39 3 -0.8946 -0.0008 -1 39 4 0.2506 -0.0010 -1 39 5 -0.7439 -0.0015 -1 40 1 0.1614 -0.0001 -1 40 2 0.6060 -0.0000 -1 40 3 0.1267 -0.0008 -1 40 4 1.0857 0.0005 -1 40 5 -0.4938 0.0016 -1 41 1 -0.2759 0.0009 -1 41 2 -0.3198 0.0019 -1 41 3 -1.0604 0.0011 -1 41 4 0.1468 -0.0005 -1 42 1 0.2922 -0.0011 -1 42 2 0.6175 -0.0027 -1 42 3 0.1566 -0.0018 -1 42 4 0.9422 -0.0013 -1 43 1 -0.2356 0.0033 -1 43 2 -0.3028 0.0032 -1 43 3 -0.7721 0.0024 -1 44 1 0.2462 -0.0019 -1 44 2 0.3222 -0.0036 0 0 2 23.8771 -0.0004 0 0 4 -2.6701 -0.0100 0 0 6 2.0397 0.0060 0 0 8 3.4035 0.0208 0 0 10 0.3849 0.0097 0 1 2 0.2316 0.0280 0 1 3 -5.3918 0.0046 0 1 4 -0.7640 0.0094 0 1 5 1.9534 0.0039 0 1 6 -1.2441 0.0198 0 1 7 -3.9313 -0.0139 0 1 9 -1.6554 -0.0154 0 1 10 -0.3866 -0.0048 0 1 11 -0.0085 0.0000 0 2 1 -0.6099 -0.0193 0 2 2 21.0230 0.0081 0 2 3 0.4836 -0.0154 0 2 4 -3.0368 -0.0064 0 2 5 1.9366 -0.0069 0 2 6 1.4656 0.0042 0 2 7 2.5235 -0.0199 0 2 8 3.0937 0.0136 0 2 9 1.6622 -0.0048 0 2 10 0.5294 0.0041 0 2 11 0.1165 0.0067 0 3 1 -33.4596 -0.0159 0 3 2 0.5218 0.0191 0 3 3 -3.2609 -0.0012 0 3 4 -1.7688 0.0011 0 3 5 2.5897 0.0028 0 3 6 -2.9503 0.0099 0 3 7 -2.8899 -0.0072 0 3 8 -3.2383 0.0101 0 3 9 -1.6286 -0.0052 0 3 10 -0.9652 -0.0025 0 3 11 -0.2550 0.0028 0 4 0 32.6378 0.0154 0 4 1 -0.8326 -0.0112 0 4 2 13.9434 0.0113 0 4 3 0.6812 -0.0045 0 4 4 -3.7545 -0.0028 0 4 5 2.5167 0.0021 0 4 6 0.1367 0.0014 0 4 7 3.7810 -0.0076 0 4 8 2.3402 0.0023 0 4 9 2.6640 -0.0010 0 4 10 0.8680 -0.0029 0 4 11 0.0692 0.0025 0 5 1 -20.0410 -0.0147 0 5 2 0.4803 0.0065 0 5 3 -0.3472 -0.0030 0 5 4 -1.5479 -0.0067 0 5 5 3.2436 0.0017 0 5 6 -2.8563 0.0001 0 5 7 -1.4188 -0.0001 0 5 8 -3.9178 0.0007 0 5 9 -1.5701 0.0052 0 5 10 -1.0849 -0.0006 0 5 11 -0.5748 0.0035 0 6 0 16.4770 0.0113 0 6 1 -0.6163 -0.0027 0 6 2 6.0236 0.0076 0 6 3 0.4150 0.0044 0 6 4 -3.9899 -0.0013 0 6 5 1.3446 0.0066 0 6 6 -1.0609 -0.0006 0 6 7 3.3067 0.0011 0 6 8 1.5207 -0.0062 0 6 9 2.7083 0.0018 0 6 10 1.1728 -0.0065 0 6 11 -0.1626 -0.0008 0 7 1 -7.3936 -0.0066 0 7 2 0.2750 -0.0024 0 7 3 1.6756 -0.0008 0 7 4 -0.2263 -0.0083 0 7 5 3.1590 0.0013 0 7 6 -1.1656 -0.0029 0 7 7 -0.2796 0.0035 0 7 8 -3.2488 -0.0035 0 7 9 -1.4384 0.0094 0 7 10 -0.7687 0.0005 0 7 11 -0.7469 0.0008 0 8 0 3.5520 0.0026 0 8 1 -0.2290 0.0022 0 8 2 0.2700 0.0006 0 8 3 -0.2085 0.0062 0 8 4 -3.1371 -0.0016 0 8 5 -0.7554 0.0041 0 8 6 -1.3918 -0.0011 0 8 7 1.6439 0.0022 0 8 8 0.9145 -0.0076 0 8 9 1.9909 0.0020 0 8 10 1.2260 -0.0041 0 8 11 -0.4313 -0.0016 0 9 1 0.9684 0.0022 0 9 2 0.1314 -0.0044 0 9 3 1.9761 0.0019 0 9 4 1.2898 -0.0036 0 9 5 2.0224 0.0013 0 9 6 0.9408 0.0001 0 9 7 0.1397 0.0026 0 9 8 -1.8226 -0.0021 0 9 9 -1.1645 0.0059 0 9 10 -0.2926 0.0007 0 9 11 -0.6601 -0.0038 0 10 0 -3.8235 -0.0046 0 10 1 0.0627 0.0028 0 10 2 -2.3281 -0.0038 0 10 3 -0.7277 0.0023 0 10 4 -1.3003 -0.0017 0 10 5 -2.3795 -0.0014 0 10 6 -0.7516 -0.0007 0 10 7 -0.1582 -0.0008 0 10 8 0.5438 -0.0029 0 10 9 1.0190 0.0007 0 10 10 0.9629 0.0017 0 11 1 4.7302 0.0063 0 11 2 0.0077 -0.0017 0 11 3 0.9548 0.0016 0 11 4 1.9311 0.0023 0 11 5 0.1977 0.0014 0 11 6 2.2483 0.0033 0 11 7 -0.0172 -0.0003 0 11 8 -0.4024 0.0005 0 11 9 -0.7327 -0.0010 0 11 10 0.0214 -0.0002 0 12 0 -6.6120 -0.0062 0 12 1 0.2451 0.0010 0 12 2 -2.6944 -0.0030 0 12 3 -0.5968 -0.0022 0 12 4 0.7768 -0.0004 0 12 5 -2.6041 -0.0043 0 12 6 0.3628 -0.0004 0 12 7 -1.3253 -0.0024 0 12 8 0.2855 0.0025 0 12 9 0.2607 0.0001 0 12 10 0.5190 0.0056 0 13 1 5.6173 0.0045 0 13 2 -0.3523 0.0013 0 13 3 -0.3118 -0.0014 0 13 4 1.2666 0.0045 0 13 5 -1.5365 0.0012 0 13 6 2.3794 0.0025 0 13 7 -0.3529 -0.0019 0 13 8 0.5623 0.0011 0 13 9 -0.2589 -0.0050 0 13 10 0.0338 -0.0012 0 14 0 -6.9698 -0.0033 0 14 1 0.4753 -0.0009 0 14 2 -2.3155 0.0010 0 14 3 0.3143 -0.0035 0 14 4 2.2259 0.0015 0 14 5 -1.6378 -0.0022 0 14 6 1.3063 -0.0009 0 14 7 -1.7916 -0.0007 0 14 8 0.0941 0.0042 0 14 9 -0.1243 0.0005 0 14 10 0.1349 0.0042 0 15 1 5.3488 0.0003 0 15 2 -1.0313 0.0020 0 15 3 -0.9555 -0.0042 0 15 4 -0.1397 0.0023 0 15 5 -2.5127 0.0010 0 15 6 1.9078 -0.0013 0 15 7 -0.6135 -0.0012 0 15 8 1.0921 0.0001 0 15 9 0.0493 -0.0036 0 15 10 -0.1350 -0.0013 0 16 0 -6.2850 0.0001 0 16 1 0.8037 -0.0015 0 16 2 -2.0185 0.0037 0 16 3 1.4746 -0.0015 0 16 4 2.5895 0.0022 0 16 5 -0.5429 0.0019 0 16 6 1.7489 -0.0016 0 16 7 -1.9979 0.0016 0 16 8 0.0735 0.0022 0 16 9 -0.2896 0.0005 0 16 10 -0.0212 -0.0006 0 17 1 4.5465 -0.0020 0 17 2 -1.6997 0.0008 0 17 3 -0.8056 -0.0037 0 17 4 -1.1744 -0.0015 0 17 5 -2.5622 0.0009 0 17 6 1.6891 -0.0038 0 17 7 -0.8307 0.0005 0 17 8 1.4500 -0.0001 0 17 9 0.0561 0.0003 0 17 10 -0.2334 -0.0004 0 18 0 -4.7892 0.0010 0 18 1 1.0569 -0.0011 0 18 2 -1.7555 0.0025 0 18 3 2.0550 0.0013 0 18 4 2.0165 0.0008 0 18 5 -0.2861 0.0041 0 18 6 1.7930 -0.0015 0 18 7 -2.3239 0.0012 0 18 8 0.3210 -0.0006 0 18 9 -0.4767 -0.0004 0 18 10 0.0265 -0.0039 0 19 1 3.0775 -0.0010 0 19 2 -1.8672 -0.0004 0 19 3 -0.2558 -0.0003 0 19 4 -1.0904 -0.0035 0 19 5 -2.0138 0.0007 0 19 6 2.0573 -0.0024 0 19 7 -1.1348 0.0011 0 19 8 1.7926 0.0015 0 19 9 -0.1612 0.0023 0 19 10 -0.1025 0.0007 0 20 0 -2.4027 -0.0003 0 20 1 1.0231 -0.0006 0 20 2 -1.1770 -0.0008 0 20 3 1.6395 0.0024 0 20 4 1.0579 -0.0012 0 20 5 -0.9531 0.0028 0 20 6 1.7262 -0.0005 0 20 7 -2.7089 -0.0017 0 20 8 0.7347 -0.0010 0 20 9 -0.7692 -0.0013 0 20 10 0.1010 -0.0027 0 21 1 0.9424 0.0009 0 21 2 -1.3847 -0.0003 0 21 3 0.1891 0.0029 0 21 4 -0.0940 -0.0028 0 21 5 -1.3694 0.0002 0 21 6 2.6042 0.0014 0 21 7 -1.4959 0.0001 0 21 8 2.0206 0.0028 0 21 9 -0.3507 0.0005 0 22 1 0.7127 -0.0007 0 22 2 -0.2131 -0.0028 0 22 3 0.6026 0.0015 0 22 4 0.2689 -0.0019 0 22 5 -1.8018 -0.0002 0 22 6 1.6992 0.0009 0 22 7 -2.7759 -0.0040 0 22 8 1.0257 0.0008 0 22 9 -1.0323 -0.0006 0 23 1 -1.3261 0.0012 0 23 2 -0.6361 0.0008 0 23 3 0.2790 0.0032 0 23 4 0.9235 -0.0009 0 23 5 -0.9412 -0.0005 0 23 6 2.6750 0.0039 0 23 7 -1.6881 -0.0013 0 23 8 1.9244 0.0018 0 23 9 -0.2969 -0.0028 0 24 1 0.3809 -0.0012 0 24 2 0.8167 -0.0017 0 24 3 -0.2449 0.0000 0 24 4 -0.1047 -0.0010 0 24 5 -2.0362 -0.0020 0 24 6 1.6260 0.0015 0 24 7 -2.2725 -0.0031 0 24 8 0.9535 0.0026 0 24 9 -1.0636 0.0013 0 25 1 -2.9618 -0.0004 0 25 2 -0.1882 0.0017 0 25 3 0.1052 0.0010 0 25 4 1.2276 0.0003 0 25 5 -0.7171 -0.0009 0 25 6 2.0409 0.0032 0 25 7 -1.5074 -0.0016 0 25 8 1.4362 -0.0012 0 25 9 -0.0119 -0.0041 0 26 0 4.2376 0.0014 0 26 1 0.2805 -0.0015 0 26 2 1.4696 0.0007 0 26 3 -0.3931 -0.0007 0 26 4 -0.1767 0.0004 0 26 5 -1.5265 -0.0016 0 26 6 1.3488 0.0008 0 26 7 -1.3606 0.0003 0 26 8 0.5507 0.0022 0 26 9 -0.7942 0.0026 0 27 1 -3.4721 -0.0019 0 27 2 -0.2645 0.0014 0 27 3 -0.0531 -0.0011 0 27 4 0.8414 0.0003 0 27 5 -0.5076 -0.0003 0 27 6 1.0961 0.0002 0 27 7 -0.9979 -0.0004 0 27 8 0.7326 -0.0036 0 27 9 0.2812 -0.0022 0 28 0 4.1170 0.0020 0 28 1 0.4192 -0.0008 0 28 2 1.4882 0.0018 0 28 3 -0.0261 -0.0004 0 28 4 -0.2133 0.0006 0 28 5 -0.8231 0.0002 0 28 6 0.8617 -0.0004 0 28 7 -0.4902 0.0033 0 28 8 0.1023 0.0000 0 29 1 -2.8841 -0.0015 0 29 2 -0.5870 0.0002 0 29 3 0.0156 -0.0011 0 29 4 0.3761 -0.0003 0 29 5 -0.2036 0.0004 0 29 6 0.4523 -0.0025 0 29 7 -0.4428 0.0009 0 29 8 0.1074 -0.0033 0 30 0 2.9340 0.0010 0 30 1 0.5800 0.0006 0 30 2 0.9523 0.0007 0 30 3 0.2752 0.0004 0 30 4 -0.3484 -0.0001 0 30 5 -0.5453 0.0015 0 30 6 0.3591 -0.0006 0 30 7 -0.0233 0.0038 0 30 8 -0.1068 -0.0022 0 31 1 -1.6641 0.0000 0 31 2 -0.7153 -0.0011 0 31 3 0.2635 0.0003 0 31 4 0.3545 -0.0006 0 31 5 0.0970 0.0001 0 31 6 0.3888 -0.0028 0 31 7 -0.1282 0.0011 0 31 8 -0.2378 -0.0007 0 32 0 1.3777 -0.0001 0 32 1 0.5598 0.0016 0 32 2 0.2428 -0.0010 0 32 3 0.1470 0.0007 0 32 4 -0.4605 -0.0003 0 32 5 -0.8091 0.0013 0 32 6 0.0739 0.0008 0 32 7 0.0111 0.0014 0 33 1 -0.4634 0.0008 0 33 2 -0.4883 -0.0015 0 33 3 0.4028 0.0012 0 33 4 0.7435 -0.0002 0 33 5 0.1946 -0.0015 0 33 6 0.6878 -0.0009 0 33 7 -0.1165 0.0001 0 34 0 0.1450 0.0004 0 34 1 0.3604 0.0015 0 34 2 -0.1679 -0.0016 0 34 3 -0.2637 0.0004 0 34 4 -0.3191 0.0006 0 34 5 -1.2217 -0.0001 0 34 6 0.0754 0.0027 0 35 1 0.1891 0.0000 0 35 2 -0.1189 -0.0009 0 35 3 0.1575 0.0009 0 35 4 1.1011 0.0004 0 35 5 0.0080 -0.0032 0 35 6 0.9309 0.0020 0 36 0 -0.3603 0.0017 0 36 1 0.1484 0.0004 0 36 2 -0.0235 -0.0009 0 36 3 -0.5505 0.0001 0 36 4 0.1389 0.0015 0 36 5 -1.3358 -0.0014 0 37 1 0.1535 -0.0010 0 37 2 0.0874 0.0000 0 37 3 -0.4475 0.0004 0 37 4 1.0743 0.0002 0 37 5 -0.3165 -0.0030 0 38 0 -0.2028 0.0021 0 38 1 0.0647 -0.0010 0 38 2 0.5140 -0.0005 0 38 3 -0.4910 0.0004 0 38 4 0.6832 0.0010 0 38 5 -1.0442 -0.0012 0 39 1 -0.2628 -0.0006 0 39 2 0.0413 0.0007 0 39 3 -1.0480 0.0008 0 39 4 0.6993 -0.0012 0 40 0 0.1796 0.0004 0 40 1 0.0996 -0.0018 0 40 2 0.9780 -0.0012 0 40 3 -0.2115 0.0011 0 40 4 0.9613 -0.0008 0 40 5 -0.5698 0.0007 0 41 1 -0.5633 0.0012 0 41 2 -0.1000 0.0011 0 41 3 -1.2309 0.0016 0 41 4 0.2709 -0.0031 0 42 0 0.3388 -0.0024 0 42 1 0.1394 -0.0021 0 42 2 0.9859 -0.0019 0 42 3 0.0156 0.0017 0 42 4 0.8100 -0.0021 0 43 1 -0.4712 0.0029 0 43 2 -0.1417 0.0016 0 43 3 -0.8969 0.0012 0 44 0 0.1689 -0.0041 0 44 1 0.0986 -0.0023 1 0 0 37.4270 0.0095 1 0 2 5.9317 0.0096 1 0 4 -1.4760 0.0028 1 0 6 5.4616 0.0096 1 0 8 2.6552 0.0110 1 0 10 0.2150 -0.0002 1 1 0 -0.9150 0.0206 1 1 1 -21.2969 -0.0151 1 1 2 -0.3351 0.0279 1 1 3 2.4140 -0.0038 1 1 4 -0.7457 0.0099 1 1 5 -2.7238 -0.0040 1 1 6 -1.0951 0.0273 1 1 7 -4.7540 -0.0095 1 1 8 -0.7634 0.0150 1 1 9 -0.9347 -0.0037 1 1 10 -0.1256 -0.0073 1 2 0 32.9025 0.0128 1 2 1 0.9187 -0.0291 1 2 2 4.3323 0.0096 1 2 3 0.9231 -0.0109 1 2 4 -1.9308 0.0008 1 2 5 1.7615 -0.0143 1 2 6 4.8846 0.0046 1 2 7 1.9942 -0.0220 1 2 8 2.6649 0.0052 1 2 9 0.7128 -0.0008 1 2 10 0.3779 -0.0029 1 3 0 -2.5961 0.0133 1 3 1 -15.4012 -0.0126 1 3 2 -0.9465 0.0170 1 3 3 3.5340 -0.0019 1 3 4 -1.6981 0.0025 1 3 5 -1.6562 -0.0004 1 3 6 -2.7583 0.0161 1 3 7 -4.1620 -0.0026 1 3 8 -2.0225 0.0081 1 3 9 -1.2607 0.0015 1 3 10 -0.2384 -0.0044 1 4 0 21.6908 0.0102 1 4 1 1.8591 -0.0146 1 4 2 0.6185 0.0049 1 4 3 1.2536 -0.0003 1 4 4 -2.8457 -0.0015 1 4 5 2.4232 -0.0036 1 4 6 3.4855 -0.0000 1 4 7 3.2515 -0.0077 1 4 8 2.6294 -0.0020 1 4 9 1.0959 0.0007 1 4 10 0.7184 -0.0051 1 5 0 -3.8130 0.0047 1 5 1 -6.8437 -0.0054 1 5 2 -1.3327 0.0024 1 5 3 4.6916 0.0015 1 5 4 -1.3916 -0.0058 1 5 5 -0.2816 0.0013 1 5 6 -3.1507 0.0019 1 5 7 -3.2293 0.0025 1 5 8 -2.6150 -0.0014 1 5 9 -1.6170 0.0055 1 5 10 -0.0585 -0.0015 1 6 0 9.1685 0.0044 1 6 1 2.6104 -0.0010 1 6 2 -2.8130 -0.0014 1 6 3 0.7426 0.0079 1 6 4 -3.2448 -0.0026 1 6 5 1.6028 0.0047 1 6 6 2.0227 -0.0010 1 6 7 3.4105 0.0048 1 6 8 2.4199 -0.0057 1 6 9 1.0367 0.0026 1 6 10 0.9275 -0.0045 1 7 0 -4.2754 -0.0009 1 7 1 0.2653 0.0016 1 7 2 -1.3222 -0.0065 1 7 3 4.6324 0.0039 1 7 4 0.0364 -0.0084 1 7 5 0.4550 0.0003 1 7 6 -2.2598 -0.0063 1 7 7 -2.2996 0.0028 1 7 8 -2.4726 -0.0072 1 7 9 -1.6684 0.0052 1 7 10 0.3073 -0.0000 1 8 0 0.0745 -0.0008 1 8 1 2.8459 0.0051 1 8 2 -4.0661 -0.0047 1 8 3 -0.2957 0.0083 1 8 4 -2.4319 -0.0020 1 8 5 -0.1266 0.0057 1 8 6 1.1532 0.0012 1 8 7 2.6372 0.0091 1 8 8 1.9752 -0.0039 1 8 9 0.7001 0.0033 1 8 10 0.8140 -0.0004 1 9 0 -3.8812 -0.0024 1 9 1 3.6367 0.0044 1 9 2 -0.9720 -0.0064 1 9 3 2.9560 0.0033 1 9 4 1.6483 -0.0042 1 9 5 0.1213 -0.0014 1 9 6 -0.7462 -0.0059 1 9 7 -1.6065 -0.0006 1 9 8 -1.8536 -0.0070 1 9 9 -1.3202 0.0006 1 9 10 0.5772 -0.0003 1 10 0 -4.0825 -0.0030 1 10 1 2.4837 0.0041 1 10 2 -2.9752 -0.0032 1 10 3 -1.0935 0.0024 1 10 4 -0.5668 -0.0005 1 10 5 -1.6606 0.0014 1 10 6 1.0183 0.0035 1 10 7 1.4598 0.0060 1 10 8 1.3775 0.0010 1 10 9 0.3853 0.0027 1 10 10 0.4635 0.0045 1 11 0 -2.8517 -0.0017 1 11 1 3.7183 0.0027 1 11 2 -0.6729 -0.0011 1 11 3 0.4089 0.0004 1 11 4 2.3470 0.0020 1 11 5 -0.9212 -0.0018 1 11 6 0.5518 -0.0014 1 11 7 -1.1736 -0.0038 1 11 8 -1.1393 -0.0036 1 11 9 -0.7772 -0.0043 1 11 10 0.5359 -0.0015 1 12 0 -4.7878 -0.0024 1 12 1 1.8540 0.0008 1 12 2 -0.8604 0.0010 1 12 3 -0.9398 -0.0035 1 12 4 1.4361 0.0004 1 12 5 -2.1629 -0.0025 1 12 6 1.2425 0.0032 1 12 7 0.3982 0.0010 1 12 8 0.8059 0.0045 1 12 9 0.2842 0.0021 1 12 10 0.1412 0.0064 1 13 0 -1.6631 -0.0007 1 13 1 2.4774 -0.0006 1 13 2 -0.8666 0.0028 1 13 3 -1.7202 -0.0025 1 13 4 1.6870 0.0046 1 13 5 -1.8450 -0.0000 1 13 6 1.1875 0.0016 1 13 7 -0.8756 -0.0039 1 13 8 -0.5723 -0.0006 1 13 9 -0.3497 -0.0055 1 13 10 0.2232 -0.0024 1 14 0 -4.3074 -0.0009 1 14 1 1.4394 -0.0009 1 14 2 0.7364 0.0042 1 14 3 0.2260 -0.0046 1 14 4 2.5687 0.0002 1 14 5 -1.6367 -0.0025 1 14 6 1.3103 0.0004 1 14 7 -0.3398 -0.0015 1 14 8 0.4125 0.0040 1 14 9 0.3357 0.0018 1 14 10 0.0478 0.0036 1 15 0 -0.7905 -0.0002 1 15 1 1.5064 -0.0025 1 15 2 -1.5928 0.0024 1 15 3 -2.5235 -0.0033 1 15 4 0.2123 0.0024 1 15 5 -1.9997 0.0022 1 15 6 1.3099 0.0013 1 15 7 -0.5918 -0.0013 1 15 8 -0.1377 0.0004 1 15 9 -0.1977 -0.0023 1 15 10 -0.0978 -0.0022 1 16 0 -3.7687 -0.0000 1 16 1 1.4522 -0.0004 1 16 2 1.1428 0.0042 1 16 3 1.6874 -0.0013 1 16 4 2.4111 -0.0006 1 16 5 -0.8048 0.0005 1 16 6 0.9867 -0.0021 1 16 7 -0.8660 -0.0015 1 16 8 0.2277 0.0008 1 16 9 0.3026 0.0015 1 17 0 -0.4646 0.0002 1 17 1 1.0995 -0.0019 1 17 2 -2.3786 -0.0003 1 17 3 -1.9870 -0.0018 1 17 4 -1.0064 -0.0016 1 17 5 -1.3560 0.0028 1 17 6 1.3614 -0.0003 1 17 7 -0.3094 0.0011 1 17 8 0.3182 0.0005 1 17 9 -0.2361 0.0020 1 18 0 -2.9541 -0.0001 1 18 1 1.7056 0.0002 1 18 2 0.7112 0.0015 1 18 3 2.5072 0.0023 1 18 4 1.3357 -0.0009 1 18 5 -0.4125 0.0025 1 18 6 0.4450 -0.0022 1 18 7 -1.3491 -0.0010 1 18 8 0.1615 -0.0016 1 18 9 0.0104 0.0007 1 19 0 -0.6250 0.0010 1 19 1 0.6902 0.0000 1 19 2 -2.6600 -0.0018 1 19 3 -0.8184 0.0003 1 19 4 -1.2649 -0.0036 1 19 5 -0.4340 0.0011 1 19 6 1.5762 -0.0003 1 19 7 -0.0979 0.0013 1 19 8 0.8515 0.0006 1 19 9 -0.2558 0.0035 1 20 0 -1.3562 -0.0006 1 20 1 1.8871 -0.0005 1 20 2 0.2180 -0.0013 1 20 3 2.3062 0.0032 1 20 4 0.1511 -0.0001 1 20 5 -0.5910 0.0017 1 20 6 0.0390 -0.0001 1 20 7 -1.7550 -0.0013 1 20 8 0.0882 -0.0015 1 20 9 -0.4664 0.0000 1 21 0 -1.0513 0.0016 1 21 1 -0.2031 0.0012 1 21 2 -2.3182 -0.0008 1 21 3 0.1392 0.0013 1 21 4 -0.7426 -0.0023 1 21 5 0.1683 -0.0015 1 21 6 1.7635 0.0014 1 21 7 -0.0029 -0.0003 1 21 8 1.3000 0.0005 1 21 9 -0.1234 0.0016 1 22 0 0.8964 -0.0004 1 22 1 1.8936 -0.0020 1 22 2 0.1915 -0.0021 1 22 3 1.5208 0.0015 1 22 4 -0.4896 0.0012 1 22 5 -0.8598 -0.0009 1 22 6 -0.0384 0.0020 1 22 7 -1.8514 -0.0016 1 22 8 -0.0593 0.0005 1 22 9 -0.8469 0.0001 1 23 0 -1.5189 0.0016 1 23 1 -1.4848 0.0008 1 23 2 -1.7529 0.0011 1 23 3 0.4335 0.0007 1 23 4 -0.1836 0.0002 1 23 5 0.2292 -0.0028 1 23 6 1.5647 0.0027 1 23 7 0.0174 -0.0017 1 23 8 1.4060 -0.0004 1 23 9 0.1195 -0.0014 1 24 0 3.0368 0.0005 1 24 1 1.8550 -0.0026 1 24 2 0.6455 -0.0010 1 24 3 0.8932 -0.0005 1 24 4 -0.4721 0.0017 1 24 5 -0.7122 -0.0028 1 24 6 0.1020 0.0022 1 24 7 -1.4634 -0.0007 1 24 8 -0.2491 0.0020 1 24 9 -0.8839 0.0009 1 25 0 -1.8641 0.0008 1 25 1 -2.6512 -0.0005 1 25 2 -1.4213 0.0018 1 25 3 0.1691 -0.0003 1 25 4 -0.1037 0.0015 1 25 5 -0.0107 -0.0019 1 25 6 0.8880 0.0023 1 25 7 0.0486 -0.0016 1 25 8 1.0634 -0.0017 1 26 0 4.2733 0.0014 1 26 1 1.8803 -0.0016 1 26 2 1.2176 0.0005 1 26 3 0.7377 -0.0008 1 26 4 -0.1641 0.0009 1 26 5 -0.1583 -0.0023 1 26 6 0.1950 0.0008 1 26 7 -0.7022 0.0011 1 26 8 -0.3861 0.0020 1 27 0 -1.9845 -0.0002 1 27 1 -3.2121 -0.0013 1 27 2 -1.3669 0.0007 1 27 3 -0.2034 -0.0005 1 27 4 -0.3369 0.0008 1 27 5 -0.1427 0.0001 1 27 6 0.0582 0.0001 1 27 7 0.1273 -0.0005 1 27 8 0.4453 -0.0023 1 28 0 4.2903 0.0014 1 28 1 1.8737 0.0002 1 28 2 1.4817 0.0009 1 28 3 0.7368 0.0003 1 28 4 -0.0265 -0.0006 1 28 5 0.3188 -0.0000 1 28 6 0.0845 -0.0008 1 28 7 0.0751 0.0025 1 28 8 -0.3930 0.0008 1 29 0 -1.8458 -0.0010 1 29 1 -2.9718 -0.0007 1 29 2 -1.2497 -0.0008 1 29 3 -0.2793 0.0002 1 29 4 -0.3371 -0.0007 1 29 5 0.0336 0.0016 1 29 6 -0.4645 -0.0022 1 29 7 0.2064 0.0005 1 29 8 -0.1145 -0.0015 1 30 0 3.3135 0.0004 1 30 1 1.6469 0.0014 1 30 2 1.2383 -0.0001 1 30 3 0.4187 0.0010 1 30 4 -0.2274 -0.0014 1 30 5 0.2921 0.0019 1 30 6 -0.1547 -0.0012 1 30 7 0.5318 0.0026 1 31 0 -1.5026 -0.0010 1 31 1 -2.0970 0.0007 1 31 2 -0.8001 -0.0010 1 31 3 -0.0040 0.0009 1 31 4 0.1621 -0.0012 1 31 5 0.3764 0.0011 1 31 6 -0.4832 -0.0030 1 31 7 0.2135 0.0009 1 32 0 1.8947 -0.0005 1 32 1 1.1686 0.0011 1 32 2 0.6536 -0.0013 1 32 3 -0.2634 0.0001 1 32 4 -0.5529 -0.0006 1 32 5 -0.1843 0.0020 1 32 6 -0.3250 -0.0003 1 32 7 0.5809 0.0014 1 33 0 -1.0782 -0.0002 1 33 1 -1.0361 0.0018 1 33 2 -0.1535 0.0002 1 33 3 0.3201 0.0007 1 33 4 0.8593 0.0002 1 33 5 0.5842 -0.0008 1 33 6 -0.1805 -0.0017 1 34 0 0.6459 -0.0006 1 34 1 0.6354 -0.0002 1 34 2 0.1524 -0.0018 1 34 3 -0.8808 -0.0017 1 34 4 -0.6532 0.0014 1 34 5 -0.6741 -0.0001 1 34 6 -0.3054 0.0007 1 35 0 -0.6897 0.0010 1 35 1 -0.2991 0.0018 1 35 2 0.2973 0.0014 1 35 3 0.3281 -0.0003 1 35 4 1.2250 0.0022 1 35 5 0.4909 -0.0028 1 35 6 0.1164 0.0009 1 36 0 -0.0141 0.0002 1 36 1 0.2835 -0.0012 1 36 2 0.0895 -0.0014 1 36 3 -1.0051 -0.0025 1 36 4 -0.3847 0.0031 1 36 5 -0.8117 -0.0027 1 36 6 -0.1449 0.0010 1 37 0 -0.3847 0.0018 1 37 1 -0.1488 0.0011 1 37 2 0.3241 0.0012 1 37 3 -0.0595 -0.0011 1 37 4 1.0395 0.0031 1 37 5 0.1984 -0.0033 1 38 0 -0.0504 0.0010 1 38 1 0.1689 -0.0010 1 38 2 0.4446 -0.0009 1 38 3 -0.6408 -0.0011 1 38 4 0.0611 0.0031 1 38 5 -0.5998 -0.0039 1 39 0 -0.1509 0.0016 1 39 1 -0.4177 0.0005 1 39 2 0.0744 -0.0005 1 39 3 -0.5498 -0.0009 1 39 4 0.5468 0.0016 1 39 5 -0.0462 -0.0020 1 40 0 0.2036 0.0008 1 40 1 0.1575 -0.0002 1 40 2 0.8318 -0.0005 1 40 3 -0.1682 0.0017 1 40 4 0.3444 0.0015 1 41 0 0.0239 0.0009 1 41 1 -0.6603 0.0001 1 41 2 -0.1258 -0.0023 1 41 3 -0.7450 -0.0003 1 41 4 0.1381 -0.0013 1 42 0 0.3317 -0.0003 1 42 1 0.1015 0.0001 1 42 2 0.8519 0.0001 1 42 3 0.0687 0.0041 1 43 0 0.1219 0.0003 1 43 1 -0.5541 -0.0001 1 43 2 -0.1054 -0.0025 1 44 0 0.1797 -0.0015 1 44 1 -0.0181 -0.0006 2 0 0 11.6475 0.0363 2 0 2 -2.1816 0.0136 2 0 4 2.4601 -0.0047 2 0 6 3.7625 -0.0014 2 0 8 0.4612 0.0038 2 1 0 -0.1838 0.0362 2 1 1 -2.1346 -0.0286 2 1 2 0.4103 0.0201 2 1 3 1.1533 -0.0002 2 1 4 -0.0806 0.0151 2 1 5 -4.3289 0.0062 2 1 6 -0.5271 0.0289 2 1 7 -1.8845 -0.0016 2 1 8 -0.2432 0.0003 2 1 9 -0.1210 -0.0020 2 1 10 -0.1151 -0.0125 2 2 0 9.1620 0.0291 2 2 1 -0.4471 -0.0303 2 2 2 -2.8196 0.0116 2 2 3 -0.4653 -0.0076 2 2 4 2.0584 -0.0064 2 2 5 0.7419 -0.0219 2 2 6 3.5513 -0.0036 2 2 7 0.8511 -0.0136 2 2 8 0.6481 0.0019 2 2 9 0.2015 0.0095 2 2 10 0.3153 0.0005 2 3 0 -0.8515 0.0220 2 3 1 0.4461 -0.0182 2 3 2 0.9470 0.0114 2 3 3 1.7789 0.0010 2 3 4 -0.1513 0.0075 2 3 5 -3.5970 0.0063 2 3 6 -1.4496 0.0162 2 3 7 -1.9426 0.0008 2 3 8 -0.6252 -0.0014 2 3 9 -0.4103 0.0007 2 3 10 -0.2004 -0.0071 2 4 0 3.3638 0.0122 2 4 1 -0.2028 -0.0133 2 4 2 -4.0980 0.0046 2 4 3 -0.8114 0.0009 2 4 4 1.1627 -0.0045 2 4 5 1.2030 -0.0083 2 4 6 2.9992 -0.0031 2 4 7 1.5048 -0.0029 2 4 8 1.0324 -0.0017 2 4 9 0.1736 0.0043 2 4 10 0.3893 -0.0026 2 5 0 -2.0373 0.0046 2 5 1 3.6411 -0.0032 2 5 2 0.9056 -0.0015 2 5 3 2.3396 0.0016 2 5 4 0.0154 -0.0020 2 5 5 -2.5495 0.0019 2 5 6 -2.0171 0.0011 2 5 7 -1.9185 0.0022 2 5 8 -0.7694 -0.0029 2 5 9 -0.7068 0.0042 2 5 10 0.0154 -0.0002 2 6 0 -2.1262 -0.0032 2 6 1 0.7160 0.0027 2 6 2 -4.6894 -0.0022 2 6 3 -1.0463 0.0076 2 6 4 0.4498 0.0001 2 6 5 1.2220 0.0030 2 6 6 2.3162 0.0004 2 6 7 1.8406 0.0054 2 6 8 1.2555 -0.0045 2 6 9 -0.1025 -0.0007 2 6 10 0.3347 -0.0046 2 7 0 -3.2260 -0.0054 2 7 1 5.1758 0.0068 2 7 2 0.4916 -0.0086 2 7 3 2.0849 0.0007 2 7 4 0.4234 -0.0061 2 7 5 -1.7269 -0.0043 2 7 6 -2.1321 -0.0074 2 7 7 -1.6937 0.0015 2 7 8 -0.7103 -0.0025 2 7 9 -0.7249 0.0055 2 7 10 0.4113 0.0037 2 8 0 -4.5447 -0.0089 2 8 1 1.6333 0.0081 2 8 2 -3.7625 -0.0043 2 8 3 -1.1944 0.0069 2 8 4 0.4114 0.0045 2 8 5 0.8689 0.0061 2 8 6 1.7366 0.0046 2 8 7 1.8654 0.0070 2 8 8 1.1131 -0.0043 2 8 9 -0.4132 -0.0032 2 9 0 -3.6108 -0.0054 2 9 1 4.2529 0.0072 2 9 2 0.0680 -0.0058 2 9 3 0.8958 -0.0012 2 9 4 0.8312 -0.0032 2 9 5 -1.4117 -0.0078 2 9 6 -1.8800 -0.0068 2 9 7 -1.3074 -0.0007 2 9 8 -0.6096 -0.0009 2 9 9 -0.4458 0.0032 2 10 0 -3.7713 -0.0056 2 10 1 1.9324 0.0037 2 10 2 -1.6879 -0.0015 2 10 3 -1.0986 0.0003 2 10 4 0.9521 0.0053 2 10 5 0.4394 0.0024 2 10 6 1.3752 0.0061 2 10 7 1.6917 0.0036 2 10 8 0.7219 -0.0014 2 10 9 -0.5009 -0.0023 2 11 0 -2.8716 -0.0005 2 11 1 1.9229 0.0015 2 11 2 -0.3010 0.0018 2 11 3 -0.5717 -0.0022 2 11 4 0.8446 0.0024 2 11 5 -1.4363 -0.0059 2 11 6 -1.4713 -0.0018 2 11 7 -0.9145 -0.0023 2 11 8 -0.6048 -0.0000 2 11 9 -0.1145 -0.0007 2 12 0 -1.7383 0.0003 2 12 1 1.6464 -0.0028 2 12 2 0.3216 0.0024 2 12 3 -0.4852 -0.0057 2 12 4 1.4619 0.0020 2 12 5 0.2491 -0.0019 2 12 6 1.1436 0.0038 2 12 7 1.4317 0.0001 2 12 8 0.3718 0.0016 2 12 9 -0.2973 0.0009 2 13 0 -1.5028 0.0024 2 13 1 -0.0764 -0.0037 2 13 2 -0.8545 0.0065 2 13 3 -1.3941 -0.0012 2 13 4 0.2504 0.0049 2 13 5 -1.3373 -0.0003 2 13 6 -1.0708 0.0016 2 13 7 -0.6239 -0.0021 2 13 8 -0.6698 -0.0009 2 13 9 0.0109 -0.0028 2 14 0 -0.3896 0.0030 2 14 1 1.3238 -0.0045 2 14 2 1.2141 0.0038 2 14 3 0.6788 -0.0061 2 14 4 1.3044 -0.0027 2 14 5 0.3572 -0.0025 2 14 6 0.8276 -0.0002 2 14 7 1.0928 -0.0007 2 14 8 0.2446 0.0024 2 14 9 0.0100 0.0036 2 15 0 -0.4017 0.0014 2 15 1 -0.7698 -0.0045 2 15 2 -1.7094 0.0047 2 15 3 -1.0799 0.0009 2 15 4 -0.7061 0.0024 2 15 5 -0.7515 0.0043 2 15 6 -0.6703 0.0015 2 15 7 -0.4079 -0.0008 2 15 8 -0.6251 -0.0025 2 15 9 -0.1123 -0.0018 2 16 0 -0.2067 0.0017 2 16 1 1.4113 -0.0014 2 16 2 0.8251 0.0021 2 16 3 1.9587 -0.0016 2 16 4 0.3251 -0.0050 2 16 5 0.5092 -0.0001 2 16 6 0.2926 -0.0025 2 16 7 0.5941 0.0002 2 16 8 0.2857 0.0012 2 16 9 0.1424 0.0040 2 17 0 -0.1654 -0.0009 2 17 1 -0.4272 -0.0018 2 17 2 -2.5793 -0.0005 2 17 3 0.1059 0.0021 2 17 4 -1.4540 -0.0018 2 17 5 0.2631 0.0046 2 17 6 -0.1620 -0.0000 2 17 7 -0.1769 0.0001 2 17 8 -0.3097 -0.0026 2 17 9 -0.3176 0.0009 2 18 0 -0.3814 -0.0006 2 18 1 1.8632 0.0020 2 18 2 -0.1941 -0.0004 2 18 3 2.7215 0.0032 2 18 4 -1.0243 -0.0033 2 18 5 0.4090 0.0019 2 18 6 -0.3622 -0.0017 2 18 7 -0.0827 0.0006 2 18 8 0.3197 -0.0006 2 19 0 -0.7467 -0.0009 2 19 1 0.0521 0.0009 2 19 2 -3.0160 -0.0037 2 19 3 1.3960 0.0013 2 19 4 -1.5922 -0.0036 2 19 5 1.2541 0.0013 2 19 6 0.4462 -0.0002 2 19 7 0.0870 0.0002 2 19 8 0.2310 -0.0011 2 20 0 -0.0015 -0.0011 2 20 1 2.3258 0.0019 2 20 2 -1.0038 -0.0014 2 20 3 2.6910 0.0041 2 20 4 -2.0305 0.0006 2 20 5 0.0597 0.0011 2 20 6 -0.8619 0.0005 2 20 7 -0.7650 -0.0002 2 20 8 0.2468 -0.0015 2 21 0 -1.6625 0.0013 2 21 1 0.0214 0.0015 2 21 2 -2.8828 -0.0026 2 21 3 2.0851 -0.0007 2 21 4 -1.2533 -0.0018 2 21 5 1.7334 -0.0023 2 21 6 0.9241 0.0010 2 21 7 0.2969 0.0002 2 21 8 0.7320 0.0003 2 22 0 1.0905 0.0000 2 22 1 2.5594 -0.0010 2 22 2 -1.1477 -0.0008 2 22 3 2.1830 0.0017 2 22 4 -2.2426 0.0034 2 22 5 -0.2087 -0.0014 2 22 6 -0.9886 0.0013 2 22 7 -1.1526 -0.0007 2 22 8 0.1120 -0.0016 2 23 0 -2.4246 0.0032 2 23 1 -0.5539 0.0004 2 23 2 -2.4718 0.0004 2 23 3 1.9576 -0.0021 2 23 4 -0.9288 0.0013 2 23 5 1.5602 -0.0030 2 23 6 0.9817 0.0020 2 23 7 0.3597 0.0006 2 23 8 0.9077 -0.0001 2 24 0 2.3844 0.0013 2 24 1 2.5824 -0.0031 2 24 2 -0.6981 0.0003 2 24 3 1.7345 -0.0010 2 24 4 -1.7570 0.0033 2 24 5 -0.0860 -0.0031 2 24 6 -0.7681 0.0003 2 24 7 -1.0520 0.0003 2 24 8 0.0139 -0.0010 2 25 0 -2.7837 0.0026 2 25 1 -1.3177 -0.0006 2 25 2 -2.1269 0.0018 2 25 3 1.3194 -0.0017 2 25 4 -0.9301 0.0028 2 25 5 1.0197 -0.0012 2 25 6 0.5574 0.0011 2 25 7 0.2800 0.0010 2 25 8 0.6906 -0.0021 2 26 0 3.2940 0.0014 2 26 1 2.4671 -0.0023 2 26 2 -0.0448 0.0006 2 26 3 1.5345 -0.0014 2 26 4 -1.0701 0.0009 2 26 5 0.3698 -0.0024 2 26 6 -0.4349 -0.0008 2 26 7 -0.5601 0.0024 2 27 0 -2.7118 0.0002 2 27 1 -1.8849 -0.0006 2 27 2 -1.8484 0.0006 2 27 3 0.6914 -0.0001 2 27 4 -1.0777 0.0015 2 27 5 0.5538 0.0009 2 27 6 -0.0803 -0.0010 2 27 7 0.1551 0.0002 2 28 0 3.5438 0.0005 2 28 1 2.1587 0.0002 2 28 2 0.4082 -0.0000 2 28 3 1.2978 0.0003 2 28 4 -0.6586 -0.0014 2 28 5 0.7710 0.0002 2 28 6 -0.2218 -0.0005 2 28 7 -0.0033 0.0037 2 29 0 -2.3033 -0.0016 2 29 1 -2.0244 0.0002 2 29 2 -1.3679 -0.0013 2 29 3 0.4306 0.0014 2 29 4 -0.9533 -0.0010 2 29 5 0.4063 0.0013 2 29 6 -0.5445 -0.0030 2 29 7 0.0782 -0.0016 2 30 0 3.1561 -0.0008 2 30 1 1.5820 0.0016 2 30 2 0.4595 -0.0008 2 30 3 0.7021 0.0017 2 30 4 -0.6490 -0.0020 2 30 5 0.7871 0.0027 2 30 6 -0.1858 0.0011 2 31 0 -1.7286 -0.0014 2 31 1 -1.6980 0.0011 2 31 2 -0.5816 -0.0014 2 31 3 0.5344 0.0016 2 31 4 -0.4099 -0.0025 2 31 5 0.4948 0.0000 2 31 6 -0.6424 -0.0037 2 32 0 2.3147 -0.0016 2 32 1 0.8614 0.0008 2 32 2 0.1876 -0.0010 2 32 3 -0.1483 0.0010 2 32 4 -0.8170 -0.0007 2 32 5 0.4536 0.0037 2 32 6 -0.2211 0.0020 2 33 0 -1.1920 0.0002 2 33 1 -1.0719 0.0016 2 33 2 0.2123 0.0005 2 33 3 0.7259 0.0002 2 33 4 0.2461 -0.0017 2 33 5 0.5732 -0.0013 2 33 6 -0.4773 -0.0031 2 34 0 1.3160 -0.0017 2 34 1 0.3069 -0.0010 2 34 2 -0.1277 -0.0003 2 34 3 -0.7779 -0.0013 2 34 4 -0.8565 0.0016 2 34 5 0.0841 0.0026 2 34 6 -0.2036 0.0011 2 35 0 -0.8315 0.0015 2 35 1 -0.4670 0.0014 2 35 2 0.5791 0.0026 2 35 3 0.7201 -0.0019 2 35 4 0.5832 0.0006 2 35 5 0.4867 -0.0019 2 36 0 0.5124 -0.0011 2 36 1 0.1347 -0.0018 2 36 2 -0.2165 0.0008 2 36 3 -0.8360 -0.0035 2 36 4 -0.6521 0.0035 2 36 5 -0.0756 0.0002 2 37 0 -0.6321 0.0013 2 37 1 -0.1689 0.0006 2 37 2 0.4045 0.0028 2 37 3 0.4538 -0.0037 2 37 4 0.4822 0.0030 2 37 5 0.2762 -0.0020 2 38 0 0.1357 0.0000 2 38 1 0.2468 -0.0006 2 38 2 -0.0300 0.0018 2 38 3 -0.4495 -0.0036 2 38 4 -0.3313 0.0045 2 39 0 -0.4663 0.0001 2 39 1 -0.2104 -0.0005 2 39 2 0.0087 0.0008 2 39 3 0.1065 -0.0044 2 39 4 0.1986 0.0040 2 40 0 0.1295 0.0012 2 40 1 0.3423 0.0014 2 40 2 0.2309 0.0024 2 40 3 -0.0531 -0.0018 2 41 0 -0.2443 -0.0007 2 41 1 -0.3546 -0.0016 2 41 2 -0.1971 -0.0017 2 41 3 -0.0869 -0.0038 2 42 0 0.2143 0.0018 2 42 1 0.2312 0.0022 2 42 2 0.3136 0.0025 2 43 0 -0.0098 -0.0003 2 43 1 -0.3358 -0.0022 3 0 0 0.1966 0.0405 3 0 2 0.4756 -0.0027 3 0 4 2.1370 -0.0062 3 0 6 -0.0325 0.0079 3 0 8 -0.2853 0.0128 3 1 0 0.9761 0.0389 3 1 1 0.6876 -0.0169 3 1 2 1.0172 0.0098 3 1 3 -1.8336 0.0097 3 1 4 0.2434 0.0193 3 1 5 -1.1018 0.0014 3 1 6 -0.1484 0.0117 3 1 7 0.4768 -0.0114 3 1 8 -0.0885 -0.0170 3 1 9 -0.1127 -0.0080 3 2 0 -0.6684 0.0353 3 2 1 -2.0652 -0.0214 3 2 2 0.2083 -0.0022 3 2 3 -1.2399 -0.0072 3 2 4 1.9128 -0.0087 3 2 5 0.1306 -0.0182 3 2 6 -0.0272 0.0041 3 2 7 0.2178 0.0058 3 2 8 -0.1704 0.0083 3 2 9 0.1963 0.0140 3 3 0 2.1500 0.0258 3 3 1 1.4980 -0.0119 3 3 2 2.4774 0.0039 3 3 3 -1.4031 0.0090 3 3 4 0.5619 0.0110 3 3 5 -0.8559 0.0037 3 3 6 -0.4527 0.0050 3 3 7 0.2945 -0.0047 3 3 8 -0.1905 -0.0105 3 3 9 -0.2185 -0.0032 3 4 0 -2.4971 0.0171 3 4 1 -2.8036 -0.0083 3 4 2 -0.3373 -0.0025 3 4 3 -1.8550 -0.0001 3 4 4 1.3771 -0.0068 3 4 5 0.3599 -0.0075 3 4 6 -0.0288 -0.0005 3 4 7 0.3727 0.0045 3 4 8 0.0638 0.0004 3 4 9 0.2152 0.0036 3 5 0 1.6817 0.0059 3 5 1 2.3249 -0.0025 3 5 2 2.6772 -0.0043 3 5 3 -0.8534 0.0050 3 5 4 0.5334 0.0023 3 5 5 -0.5027 0.0025 3 5 6 -0.7429 -0.0007 3 5 7 0.0835 0.0028 3 5 8 -0.1228 -0.0013 3 5 9 -0.2939 0.0025 3 6 0 -3.7081 -0.0015 3 6 1 -1.9764 0.0045 3 6 2 -0.6455 -0.0022 3 6 3 -1.7071 0.0043 3 6 4 0.8471 -0.0012 3 6 5 0.6497 -0.0001 3 6 6 -0.0463 -0.0026 3 6 7 0.4248 0.0011 3 6 8 0.2037 -0.0063 3 6 9 0.0187 -0.0054 3 7 0 0.1122 -0.0070 3 7 1 2.3539 0.0039 3 7 2 1.8477 -0.0072 3 7 3 -0.5371 -0.0004 3 7 4 0.2615 -0.0012 3 7 5 -0.2533 -0.0013 3 7 6 -0.9472 -0.0019 3 7 7 -0.0183 0.0067 3 7 8 0.0846 0.0057 3 7 9 -0.2210 0.0057 3 8 0 -3.3422 -0.0097 3 8 1 -0.4667 0.0077 3 8 2 -0.4515 -0.0003 3 8 3 -1.1130 0.0025 3 8 4 0.5904 0.0043 3 8 5 0.8730 0.0012 3 8 6 -0.0277 -0.0016 3 8 7 0.3857 -0.0027 3 8 8 0.1520 -0.0082 3 8 9 -0.2714 -0.0083 3 9 0 -1.2238 -0.0070 3 9 1 1.5184 0.0037 3 9 2 0.7154 -0.0025 3 9 3 -0.5343 -0.0039 3 9 4 -0.0662 0.0007 3 9 5 -0.2497 -0.0045 3 9 6 -1.0188 0.0004 3 9 7 -0.0235 0.0060 3 9 8 0.3022 0.0075 3 9 9 -0.0335 0.0050 3 10 0 -1.8186 -0.0067 3 10 1 0.6733 0.0015 3 10 2 -0.0127 0.0020 3 10 3 -0.3997 -0.0028 3 10 4 0.6066 0.0056 3 10 5 0.9798 -0.0011 3 10 6 0.0908 0.0003 3 10 7 0.3201 -0.0042 3 10 8 0.0097 -0.0056 3 10 9 -0.4837 -0.0051 3 11 0 -1.4459 0.0006 3 11 1 0.5206 -0.0007 3 11 2 -0.2476 0.0048 3 11 3 -0.5628 -0.0033 3 11 4 -0.4204 0.0035 3 11 5 -0.4226 -0.0039 3 11 6 -0.9936 0.0023 3 11 7 -0.0431 0.0028 3 11 8 0.4026 0.0041 3 12 0 -0.3736 0.0004 3 12 1 1.1176 -0.0059 3 12 2 0.1148 0.0027 3 12 3 0.3887 -0.0061 3 12 4 0.5978 0.0019 3 12 5 1.0472 -0.0023 3 12 6 0.2699 0.0008 3 12 7 0.2933 -0.0024 3 12 8 -0.0540 -0.0016 3 13 0 -0.7807 0.0058 3 13 1 0.1443 -0.0041 3 13 2 -1.0775 0.0078 3 13 3 -0.2073 0.0005 3 13 4 -0.8917 0.0031 3 13 5 -0.4965 -0.0003 3 13 6 -0.9370 0.0017 3 13 7 -0.1293 0.0001 3 13 8 0.3588 -0.0013 3 14 0 0.1261 0.0042 3 14 1 1.2643 -0.0071 3 14 2 -0.4255 0.0011 3 14 3 1.3141 -0.0041 3 14 4 0.2012 -0.0034 3 14 5 1.1392 -0.0009 3 14 6 0.3484 0.0001 3 14 7 0.2994 0.0010 3 14 8 0.0219 0.0007 3 15 0 -0.1171 0.0041 3 15 1 0.5759 -0.0036 3 15 2 -1.9320 0.0043 3 15 3 0.7097 0.0042 3 15 4 -1.4401 -0.0003 3 15 5 -0.2080 0.0029 3 15 6 -0.8391 -0.0004 3 15 7 -0.2150 -0.0011 3 15 8 0.2545 -0.0045 3 16 0 -0.1940 0.0030 3 16 1 1.5520 -0.0021 3 16 2 -1.4770 -0.0013 3 16 3 2.2100 0.0009 3 16 4 -0.6734 -0.0057 3 16 5 1.1662 0.0014 3 16 6 0.1946 -0.0003 3 16 7 0.2528 0.0029 3 16 8 0.1613 0.0009 3 17 0 -0.0944 -0.0009 3 17 1 1.3466 -0.0006 3 17 2 -2.6706 -0.0018 3 17 3 1.9233 0.0047 3 17 4 -1.7982 -0.0032 3 17 5 0.4257 0.0029 3 17 6 -0.6083 -0.0012 3 17 7 -0.2201 -0.0013 3 17 8 0.1984 -0.0040 3 18 0 -0.6034 -0.0001 3 18 1 1.9662 0.0033 3 18 2 -2.4936 -0.0023 3 18 3 2.6901 0.0043 3 18 4 -1.6958 -0.0033 3 18 5 0.9583 0.0016 3 18 6 -0.1218 0.0004 3 18 7 0.0752 0.0019 3 18 8 0.2698 0.0000 3 19 0 -0.6603 -0.0034 3 19 1 1.8315 0.0018 3 19 2 -2.9498 -0.0048 3 19 3 2.8754 0.0017 3 19 4 -1.7076 -0.0028 3 19 5 1.0590 0.0002 3 19 6 -0.1977 -0.0000 3 19 7 -0.1744 -0.0008 3 20 0 -0.5631 -0.0016 3 20 1 2.2077 0.0041 3 20 2 -2.9530 -0.0013 3 20 3 2.5307 0.0035 3 20 4 -2.3276 0.0011 3 20 5 0.4894 -0.0005 3 20 6 -0.3504 0.0011 3 20 7 -0.2031 -0.0002 3 21 0 -1.3617 -0.0012 3 21 1 1.7466 0.0020 3 21 2 -2.6624 -0.0031 3 21 3 3.1082 -0.0020 3 21 4 -1.2239 0.0003 3 21 5 1.2829 -0.0020 3 21 6 0.2801 0.0015 3 21 7 -0.1917 0.0002 3 22 0 -0.0896 -0.0010 3 22 1 2.1503 0.0007 3 22 2 -2.6964 0.0005 3 22 3 1.9482 0.0001 3 22 4 -2.2404 0.0036 3 22 5 -0.0245 -0.0026 3 22 6 -0.2852 0.0002 3 22 7 -0.4436 -0.0007 3 23 0 -1.8545 0.0025 3 23 1 1.2282 0.0009 3 23 2 -2.1113 0.0003 3 23 3 2.5884 -0.0034 3 23 4 -0.7022 0.0030 3 23 5 0.9734 -0.0013 3 23 6 0.6057 0.0012 3 23 7 -0.3248 0.0018 3 24 0 0.5011 0.0002 3 24 1 1.9636 -0.0024 3 24 2 -1.9618 0.0012 3 24 3 1.3971 -0.0023 3 24 4 -1.5723 0.0025 3 24 5 -0.2975 -0.0026 3 24 6 0.0331 -0.0018 3 24 7 -0.5148 0.0013 3 25 0 -2.0734 0.0037 3 25 1 0.5781 0.0000 3 25 2 -1.6799 0.0017 3 25 3 1.7022 -0.0020 3 25 4 -0.4522 0.0031 3 25 5 0.3892 0.0010 3 25 6 0.6369 -0.0011 3 25 7 -0.4821 0.0026 3 26 0 0.9916 0.0004 3 26 1 1.8143 -0.0022 3 26 2 -1.1585 0.0006 3 26 3 1.1095 -0.0018 3 26 4 -0.7954 -0.0003 3 26 5 -0.2396 -0.0006 3 26 6 0.3563 -0.0027 3 27 0 -2.0556 0.0017 3 27 1 0.0228 -0.0001 3 27 2 -1.4173 0.0002 3 27 3 0.9480 0.0006 3 27 4 -0.4521 0.0010 3 27 5 -0.0706 0.0021 3 27 6 0.4296 -0.0034 3 28 0 1.3445 -0.0000 3 28 1 1.6149 0.0003 3 28 2 -0.6025 -0.0006 3 28 3 0.9165 0.0006 3 28 4 -0.3268 -0.0020 3 28 5 -0.0170 0.0017 3 28 6 0.4634 -0.0008 3 29 0 -1.7945 -0.0010 3 29 1 -0.3292 0.0001 3 29 2 -1.0590 -0.0019 3 29 3 0.5945 0.0020 3 29 4 -0.4411 -0.0014 3 29 5 -0.1992 0.0006 3 29 6 0.1676 -0.0038 3 30 0 1.5272 -0.0004 3 30 1 1.1718 0.0020 3 30 2 -0.3837 -0.0009 3 30 3 0.5440 0.0022 3 30 4 -0.2457 -0.0013 3 30 5 0.1451 0.0028 3 30 6 0.3440 0.0024 3 31 0 -1.3175 -0.0018 3 31 1 -0.4346 0.0000 3 31 2 -0.4408 -0.0021 3 31 3 0.5709 0.0014 3 31 4 -0.2563 -0.0026 3 31 5 -0.0908 -0.0021 3 32 0 1.4335 -0.0006 3 32 1 0.5197 0.0014 3 32 2 -0.3947 -0.0003 3 32 3 0.0008 0.0018 3 32 4 -0.3398 0.0008 3 32 5 0.1775 0.0029 3 33 0 -0.7982 -0.0009 3 33 1 -0.3148 -0.0002 3 33 2 0.2251 -0.0000 3 33 3 0.6272 -0.0003 3 33 4 -0.0058 -0.0024 3 33 5 0.0319 -0.0034 3 34 0 1.0290 -0.0006 3 34 1 -0.0227 -0.0006 3 34 2 -0.4532 0.0008 3 34 3 -0.4109 -0.0002 3 34 4 -0.3718 0.0024 3 34 5 0.1673 0.0025 3 35 0 -0.4681 0.0001 3 35 1 -0.0894 -0.0004 3 35 2 0.5551 0.0025 3 35 3 0.5775 -0.0022 3 35 4 0.1015 -0.0013 3 36 0 0.4891 -0.0004 3 36 1 -0.1704 -0.0019 3 36 2 -0.4256 0.0020 3 36 3 -0.4500 -0.0022 3 36 4 -0.2790 0.0031 3 37 0 -0.3995 -0.0001 3 37 1 0.0705 -0.0008 3 37 2 0.4214 0.0037 3 37 3 0.4126 -0.0038 3 38 0 0.0965 0.0003 3 38 1 0.0212 -0.0015 3 38 2 -0.2928 0.0032 3 38 3 -0.2102 -0.0034 3 39 0 -0.4362 -0.0010 3 39 1 0.0706 -0.0017 3 39 2 0.0854 0.0032 3 40 0 -0.0083 0.0016 3 40 1 0.2283 -0.0002 3 41 0 -0.3738 -0.0013 4 0 0 2.2217 0.0059 4 0 2 1.8281 -0.0057 4 0 4 -1.0475 0.0135 4 0 6 -1.0923 0.0230 4 1 0 1.0225 0.0274 4 1 1 -2.5027 0.0078 4 1 2 0.8116 0.0053 4 1 3 -0.2600 -0.0018 4 1 4 0.2182 0.0142 4 1 5 1.5230 -0.0160 4 1 6 -0.0360 -0.0078 4 1 7 0.4119 -0.0164 4 1 8 -0.0980 -0.0153 4 2 0 1.9053 0.0069 4 2 1 -1.8140 -0.0081 4 2 2 1.5706 -0.0082 4 2 3 -0.9454 -0.0088 4 2 4 -1.1867 0.0061 4 2 5 -0.0669 -0.0049 4 2 6 -1.0978 0.0127 4 2 7 0.1463 0.0137 4 2 8 0.0206 0.0064 4 3 0 2.3658 0.0185 4 3 1 -1.9642 0.0072 4 3 2 1.9627 -0.0001 4 3 3 0.1170 0.0037 4 3 4 0.5194 0.0098 4 3 5 1.6439 -0.0052 4 3 6 -0.1019 -0.0061 4 3 7 0.3434 -0.0048 4 3 8 -0.2641 -0.0074 4 4 0 1.2002 0.0030 4 4 1 -2.5148 0.0006 4 4 2 0.9478 -0.0089 4 4 3 -1.3839 -0.0036 4 4 4 -1.4974 -0.0016 4 4 5 -0.0719 -0.0025 4 4 6 -1.1047 0.0001 4 4 7 0.2331 0.0059 4 4 8 0.1434 -0.0008 4 5 0 2.2038 0.0032 4 5 1 -1.2132 0.0061 4 5 2 2.0937 -0.0050 4 5 3 0.6280 0.0062 4 5 4 0.5590 0.0053 4 5 5 1.7620 0.0033 4 5 6 -0.1158 -0.0025 4 5 7 0.2676 0.0049 4 5 8 -0.3371 0.0015 4 6 0 0.5945 -0.0019 4 6 1 -1.8987 0.0075 4 6 2 0.3006 -0.0068 4 6 3 -1.2449 -0.0006 4 6 4 -1.7118 -0.0045 4 6 5 -0.0687 -0.0015 4 6 6 -1.0670 -0.0070 4 6 7 0.1847 -0.0016 4 6 8 0.2088 -0.0042 4 7 0 0.9446 -0.0073 4 7 1 -0.6156 0.0037 4 7 2 1.4369 -0.0051 4 7 3 0.9360 0.0046 4 7 4 0.4646 0.0029 4 7 5 1.6829 0.0050 4 7 6 0.0059 0.0011 4 7 7 0.2236 0.0078 4 7 8 -0.2620 0.0067 4 8 0 0.3458 -0.0032 4 8 1 -0.6870 0.0070 4 8 2 -0.0895 -0.0029 4 8 3 -0.8545 -0.0011 4 8 4 -1.5648 -0.0022 4 8 5 -0.1689 -0.0016 4 8 6 -0.9027 -0.0065 4 8 7 -0.0474 -0.0054 4 8 8 0.1682 -0.0034 4 9 0 -0.3179 -0.0070 4 9 1 -0.2716 0.0001 4 9 2 0.6195 -0.0007 4 9 3 0.8479 0.0011 4 9 4 0.4171 0.0023 4 9 5 1.2737 0.0016 4 9 6 0.2862 0.0029 4 9 7 0.1791 0.0051 4 9 8 -0.0322 0.0064 4 10 0 0.2706 -0.0004 4 10 1 0.2790 0.0007 4 10 2 -0.2143 0.0004 4 10 3 -0.5033 -0.0027 4 10 4 -1.0096 0.0012 4 10 5 -0.3695 -0.0016 4 10 6 -0.5711 -0.0022 4 10 7 -0.4105 -0.0047 4 11 0 -0.8427 -0.0001 4 11 1 0.0294 -0.0028 4 11 2 0.0006 0.0038 4 11 3 0.4898 -0.0007 4 11 4 0.3967 0.0015 4 11 5 0.6163 -0.0019 4 11 6 0.6034 0.0024 4 11 7 0.0876 0.0015 4 12 0 -0.0058 0.0032 4 12 1 0.7586 -0.0049 4 12 2 -0.3384 0.0010 4 12 3 -0.1515 -0.0023 4 12 4 -0.3213 0.0019 4 12 5 -0.4952 -0.0009 4 12 6 -0.1660 0.0008 4 12 7 -0.7402 -0.0015 4 13 0 -0.7341 0.0049 4 13 1 0.5652 -0.0033 4 13 2 -0.5383 0.0041 4 13 3 0.2481 0.0006 4 13 4 0.2026 -0.0001 4 13 5 0.0163 -0.0021 4 13 6 0.7501 0.0009 4 13 7 -0.0280 0.0001 4 14 0 -0.6282 0.0042 4 14 1 1.0582 -0.0049 4 14 2 -0.7621 -0.0007 4 14 3 0.4034 0.0003 4 14 4 0.0662 -0.0002 4 14 5 -0.3619 -0.0002 4 14 6 0.1156 0.0010 4 14 7 -0.8575 0.0013 4 15 0 -0.5389 0.0037 4 15 1 1.3803 -0.0013 4 15 2 -1.2107 0.0004 4 15 3 0.4610 0.0030 4 15 4 -0.2659 -0.0015 4 15 5 -0.2144 -0.0003 4 15 6 0.6102 0.0001 4 15 7 -0.0892 0.0003 4 16 0 -1.3577 0.0022 4 16 1 1.4416 -0.0003 4 16 2 -1.5231 -0.0026 4 16 3 1.1422 0.0030 4 16 4 -0.0844 -0.0022 4 16 5 0.0048 -0.0006 4 16 6 0.1478 0.0003 4 16 7 -0.7032 0.0021 4 17 0 -0.5638 -0.0009 4 17 1 2.2035 0.0010 4 17 2 -1.9023 -0.0034 4 17 3 1.0958 0.0033 4 17 4 -0.8095 -0.0011 4 17 5 -0.0397 0.0006 4 17 6 0.2791 0.0006 4 17 7 -0.0668 0.0003 4 18 0 -1.8065 -0.0005 4 18 1 1.7733 0.0036 4 18 2 -2.3029 -0.0023 4 18 3 1.7201 0.0030 4 18 4 -0.5784 -0.0016 4 18 5 0.3456 -0.0019 4 18 6 0.0215 0.0005 4 18 7 -0.3856 0.0010 4 19 0 -0.6798 -0.0034 4 19 1 2.6442 0.0017 4 19 2 -2.2311 -0.0039 4 19 3 1.7240 0.0009 4 19 4 -1.0629 0.0009 4 19 5 0.2417 -0.0003 4 19 6 -0.0026 0.0015 4 20 0 -1.7784 -0.0018 4 20 1 1.7572 0.0035 4 20 2 -2.6442 -0.0000 4 20 3 1.7758 0.0005 4 20 4 -0.9310 0.0008 4 20 5 0.3854 -0.0028 4 20 6 -0.0225 0.0011 4 21 0 -0.6752 -0.0017 4 21 1 2.4873 0.0008 4 21 2 -1.9795 -0.0012 4 21 3 1.8590 -0.0022 4 21 4 -0.8301 0.0027 4 21 5 0.2579 -0.0011 4 21 6 -0.0488 0.0013 4 22 0 -1.3810 -0.0015 4 22 1 1.3706 0.0006 4 22 2 -2.3136 0.0021 4 22 3 1.2907 -0.0022 4 22 4 -0.7858 0.0020 4 22 5 0.0755 -0.0022 4 22 6 0.1685 0.0004 4 23 0 -0.5932 0.0014 4 23 1 1.8402 -0.0002 4 23 2 -1.3454 0.0014 4 23 3 1.3671 -0.0031 4 23 4 -0.2602 0.0029 4 23 5 -0.0943 0.0001 4 23 6 0.1290 -0.0003 4 24 0 -0.8619 -0.0008 4 24 1 0.9187 -0.0015 4 24 2 -1.4944 0.0022 4 24 3 0.5940 -0.0028 4 24 4 -0.2172 0.0006 4 24 5 -0.3752 -0.0002 4 24 6 0.4982 -0.0018 4 25 0 -0.6336 0.0025 4 25 1 1.0369 -0.0002 4 25 2 -0.7273 0.0016 4 25 3 0.5677 -0.0012 4 25 4 0.3014 0.0015 4 25 5 -0.5699 0.0023 4 25 6 0.3561 -0.0023 4 26 0 -0.3985 -0.0005 4 26 1 0.6731 -0.0008 4 26 2 -0.6405 0.0004 4 26 3 0.0413 -0.0014 4 26 4 0.3710 -0.0018 4 26 5 -0.6870 0.0016 4 27 0 -0.8226 0.0010 4 27 1 0.4077 0.0004 4 27 2 -0.3330 -0.0002 4 27 3 -0.0585 0.0015 4 27 4 0.6012 -0.0001 4 27 5 -0.8294 0.0030 4 28 0 -0.0455 -0.0002 4 28 1 0.5817 0.0012 4 28 2 -0.1311 -0.0015 4 28 3 -0.2532 0.0003 4 28 4 0.6283 -0.0024 4 28 5 -0.7170 0.0019 4 29 0 -0.9296 -0.0010 4 29 1 0.0997 0.0006 4 29 2 -0.0749 -0.0017 4 29 3 -0.2613 0.0024 4 29 4 0.6124 -0.0007 4 29 5 -0.7495 0.0008 4 30 0 0.1868 0.0003 4 30 1 0.4015 0.0020 4 30 2 -0.0320 -0.0017 4 30 3 -0.3771 0.0009 4 30 4 0.5286 -0.0005 4 31 0 -0.7445 -0.0016 4 31 1 0.0557 0.0002 4 31 2 0.1875 -0.0013 4 31 3 -0.1478 0.0010 4 31 4 0.4478 -0.0006 4 32 0 0.2771 0.0006 4 32 1 0.0519 0.0009 4 32 2 -0.1431 -0.0007 4 32 3 -0.4103 0.0005 4 32 4 0.2984 0.0023 4 33 0 -0.3489 -0.0009 4 33 1 0.1192 -0.0003 4 33 2 0.4140 0.0004 4 33 3 0.0168 -0.0011 4 34 0 0.2288 0.0002 4 34 1 -0.2690 -0.0010 4 34 2 -0.2323 0.0005 4 34 3 -0.3392 -0.0000 4 35 0 -0.0380 -0.0003 4 35 1 0.1595 -0.0002 4 35 2 0.4505 0.0019 4 36 0 0.1141 -0.0007 4 36 1 -0.3299 -0.0021 4 36 2 -0.2142 0.0011 4 37 0 0.0024 -0.0003 4 37 1 0.1313 0.0001 5 0 0 2.9218 -0.0184 5 0 2 -0.5144 0.0106 5 0 4 -1.5828 0.0198 5 0 6 -0.1369 0.0156 5 1 0 0.5525 0.0125 5 1 1 -1.3202 0.0076 5 1 2 0.5470 0.0049 5 1 3 1.6959 -0.0155 5 1 4 0.2083 0.0050 5 1 5 0.8074 -0.0135 5 1 6 -0.0748 -0.0084 5 2 0 2.6501 -0.0181 5 2 1 -1.0895 -0.0003 5 2 2 -0.7388 0.0043 5 2 3 -0.7421 -0.0085 5 2 4 -1.6656 0.0103 5 2 5 -0.0844 0.0029 5 2 6 -0.1345 0.0043 5 3 0 1.2355 0.0041 5 3 1 -0.7864 0.0096 5 3 2 1.3388 0.0019 5 3 3 1.9567 -0.0058 5 3 4 0.5550 0.0053 5 3 5 0.8797 -0.0016 5 3 6 -0.2002 -0.0054 5 4 0 1.9819 -0.0132 5 4 1 -1.4882 0.0060 5 4 2 -1.2712 -0.0026 5 4 3 -1.1719 -0.0070 5 4 4 -1.8508 0.0000 5 4 5 -0.1791 0.0016 5 4 6 -0.1388 -0.0047 5 5 0 1.0335 -0.0056 5 5 1 -0.0218 0.0088 5 5 2 1.4982 -0.0009 5 5 3 2.2821 0.0023 5 5 4 0.7812 0.0041 5 5 5 0.9720 0.0054 5 5 6 -0.2292 -0.0024 5 6 0 1.2556 -0.0060 5 6 1 -1.1133 0.0088 5 6 2 -1.7561 -0.0061 5 6 3 -1.2726 -0.0042 5 6 4 -1.9645 -0.0042 5 6 5 -0.3543 0.0014 5 6 6 -0.1557 -0.0060 5 7 0 0.2413 -0.0097 5 7 1 0.5472 0.0055 5 7 2 1.2288 -0.0017 5 7 3 2.3642 0.0046 5 7 4 0.9860 0.0012 5 7 5 0.9794 0.0042 5 7 6 -0.0704 -0.0011 5 8 0 0.7642 0.0004 5 8 1 -0.4824 0.0062 5 8 2 -1.8222 -0.0053 5 8 3 -1.2857 -0.0012 5 8 4 -1.8009 -0.0016 5 8 5 -0.6828 0.0025 5 8 6 -0.1516 -0.0014 5 9 0 -0.4490 -0.0063 5 9 1 0.6471 0.0015 5 9 2 0.9807 -0.0006 5 9 3 1.9712 0.0018 5 9 4 1.2697 -0.0020 5 9 5 0.8041 -0.0013 5 9 6 0.2962 -0.0012 5 10 0 0.5566 0.0041 5 10 1 -0.1410 0.0008 5 10 2 -1.3427 -0.0022 5 10 3 -1.3912 0.0012 5 10 4 -1.2819 0.0033 5 10 5 -1.1099 0.0032 5 10 6 -0.0864 0.0029 5 11 0 -0.6196 -0.0001 5 11 1 0.3559 -0.0009 5 11 2 0.9538 0.0002 5 11 3 1.1575 -0.0016 5 11 4 1.5500 -0.0033 5 11 5 0.4638 -0.0048 5 11 6 0.7367 -0.0011 5 12 0 0.4294 0.0043 5 12 1 -0.1563 -0.0023 5 12 2 -0.5765 -0.0002 5 12 3 -1.4779 0.0023 5 12 4 -0.5787 0.0051 5 12 5 -1.4169 0.0019 5 12 6 0.0142 0.0028 5 13 0 -0.4136 0.0030 5 13 1 0.0539 -0.0008 5 13 2 0.9319 -0.0004 5 13 3 0.2967 -0.0022 5 13 4 1.5829 -0.0017 5 13 5 0.1294 -0.0036 5 13 6 1.0104 -0.0000 5 14 0 0.1237 0.0021 5 14 1 -0.1747 -0.0012 5 14 2 -0.0143 -0.0006 5 14 3 -1.2674 0.0018 5 14 4 -0.0340 0.0030 5 14 5 -1.3690 -0.0014 5 14 6 0.0540 -0.0002 5 15 0 -0.2288 0.0013 5 15 1 0.1173 0.0008 5 15 2 0.5908 -0.0020 5 15 3 -0.1695 -0.0002 5 15 4 1.2003 0.0018 5 15 5 -0.0002 -0.0005 5 15 6 0.9428 0.0015 5 16 0 -0.4265 -0.0004 5 16 1 0.1046 0.0021 5 16 2 0.0041 -0.0018 5 16 3 -0.6537 0.0000 5 16 4 0.1092 -0.0001 5 16 5 -0.9323 -0.0047 5 16 6 -0.0332 -0.0019 5 17 0 -0.2537 -0.0021 5 17 1 0.5884 0.0019 5 17 2 -0.0948 -0.0025 5 17 3 -0.0927 0.0016 5 17 4 0.5240 0.0050 5 17 5 0.1071 0.0010 5 18 0 -1.0083 -0.0013 5 18 1 0.5966 0.0038 5 18 2 -0.4170 -0.0018 5 18 3 0.1177 -0.0020 5 18 4 -0.0706 -0.0012 5 18 5 -0.3442 -0.0057 5 19 0 -0.3549 -0.0032 5 19 1 1.1194 0.0009 5 19 2 -0.7824 -0.0012 5 19 3 0.2533 0.0013 5 19 4 -0.0791 0.0057 5 19 5 0.2649 0.0000 5 20 0 -1.2893 -0.0003 5 20 1 0.9543 0.0024 5 20 2 -0.8164 -0.0000 5 20 3 0.6221 -0.0032 5 20 4 -0.2431 -0.0005 5 20 5 0.0530 -0.0040 5 21 0 -0.3385 -0.0014 5 21 1 1.2659 -0.0010 5 21 2 -1.0693 0.0009 5 21 3 0.4233 -0.0001 5 21 4 -0.2773 0.0039 5 21 5 0.2416 -0.0009 5 22 0 -1.0939 0.0009 5 22 1 0.9340 -0.0002 5 22 2 -0.7854 0.0017 5 22 3 0.6006 -0.0029 5 22 4 -0.1382 -0.0001 5 22 5 0.0777 -0.0010 5 23 0 -0.1975 0.0008 5 23 1 0.8733 -0.0020 5 23 2 -0.8276 0.0020 5 23 3 0.2011 -0.0005 5 23 4 -0.0299 0.0012 5 24 0 -0.5552 0.0008 5 24 1 0.5854 -0.0015 5 24 2 -0.3140 0.0015 5 24 3 0.1459 -0.0017 5 24 4 0.2108 -0.0013 5 25 0 -0.0669 0.0011 5 25 1 0.2003 -0.0009 5 25 2 -0.2573 0.0016 5 25 3 -0.2424 0.0008 5 25 4 0.4053 -0.0005 5 26 0 -0.0094 -0.0004 5 26 1 0.1314 -0.0006 5 26 2 0.2452 -0.0004 5 26 3 -0.4096 -0.0007 5 26 4 0.5341 -0.0026 5 27 0 -0.0172 -0.0001 5 27 1 -0.3228 0.0011 5 27 2 0.3197 0.0005 5 27 3 -0.5632 0.0020 5 28 0 0.2661 -0.0016 5 28 1 -0.2466 0.0007 5 28 2 0.5290 -0.0020 5 28 3 -0.7538 -0.0005 5 29 0 0.0147 -0.0010 5 29 1 -0.4544 0.0022 5 29 2 0.6755 -0.0001 5 29 3 -0.5801 0.0015 5 30 0 0.2380 -0.0015 5 30 1 -0.4782 0.0010 5 30 2 0.4629 -0.0018 5 30 3 -0.7712 -0.0008 5 31 0 0.0956 -0.0007 5 31 1 -0.2850 0.0016 5 31 2 0.7441 0.0001 5 32 0 0.0818 -0.0009 5 32 1 -0.5432 0.0001 5 32 2 0.2410 -0.0004 5 33 0 0.1773 -0.0000 5 33 1 -0.0733 0.0007 5 34 0 -0.0092 -0.0009 6 0 0 -0.0439 -0.0078 6 0 2 -1.0432 0.0118 6 0 4 -0.0106 0.0034 6 1 0 0.4053 0.0024 6 1 1 0.8281 -0.0058 6 1 2 0.4572 0.0040 6 1 3 0.6276 -0.0051 6 1 4 0.1160 0.0014 6 2 0 -0.1421 -0.0100 6 2 1 -0.8856 0.0009 6 2 2 -1.1003 0.0075 6 2 3 -0.6098 -0.0056 6 2 4 0.0012 -0.0028 6 2 5 0.1177 0.0012 6 3 0 0.9242 -0.0046 6 3 1 1.0209 -0.0018 6 3 2 1.1680 0.0047 6 3 3 0.6571 -0.0003 6 3 4 0.3367 0.0016 6 3 5 -0.2820 0.0066 6 4 0 -0.3765 -0.0080 6 4 1 -1.2917 0.0033 6 4 2 -1.2567 0.0024 6 4 3 -1.0319 -0.0058 6 4 4 -0.0016 -0.0055 6 4 5 0.1504 0.0012 6 5 0 0.8295 -0.0094 6 5 1 1.2976 0.0011 6 5 2 1.4362 0.0038 6 5 3 0.7445 0.0015 6 5 4 0.5404 0.0005 6 5 5 -0.2792 0.0058 6 6 0 -0.5793 -0.0035 6 6 1 -1.1479 0.0038 6 6 2 -1.4337 -0.0004 6 6 3 -1.2266 -0.0032 6 6 4 -0.0757 -0.0024 6 6 5 0.0480 0.0022 6 7 0 0.3336 -0.0082 6 7 1 1.4481 0.0017 6 7 2 1.3672 0.0018 6 7 3 0.8602 -0.0007 6 7 4 0.7454 -0.0026 6 7 5 -0.2067 0.0001 6 8 0 -0.5471 0.0009 6 8 1 -0.8161 0.0018 6 8 2 -1.4641 0.0000 6 8 3 -1.3026 0.0012 6 8 4 -0.2043 0.0034 6 8 5 -0.1732 0.0039 6 9 0 -0.0432 -0.0025 6 9 1 1.2587 0.0007 6 9 2 1.2655 -0.0005 6 9 3 0.8872 -0.0044 6 9 4 0.9525 -0.0055 6 9 5 -0.0954 -0.0048 6 10 0 -0.1878 0.0028 6 10 1 -0.7211 -0.0006 6 10 2 -1.1925 0.0018 6 10 3 -1.3744 0.0044 6 10 4 -0.3011 0.0068 6 10 5 -0.4228 0.0044 6 11 0 0.0431 0.0026 6 11 1 0.6934 -0.0003 6 11 2 1.3235 -0.0018 6 11 3 0.7283 -0.0061 6 11 4 1.1016 -0.0054 6 12 0 0.3561 0.0018 6 12 1 -0.9577 -0.0013 6 12 2 -0.6473 0.0025 6 12 3 -1.4287 0.0039 6 12 4 -0.3144 0.0056 6 13 0 0.4809 0.0031 6 13 1 -0.0085 0.0001 6 13 2 1.4480 -0.0016 6 13 3 0.4370 -0.0044 6 13 4 1.0924 -0.0014 6 14 0 0.7645 -0.0007 6 14 1 -1.2352 0.0002 6 14 2 -0.0811 0.0010 6 14 3 -1.3401 -0.0001 6 14 4 -0.2938 0.0018 6 15 0 0.8529 -0.0003 6 15 1 -0.4739 0.0016 6 15 2 1.3788 -0.0001 6 15 3 0.1968 -0.0010 6 15 4 0.8710 0.0042 6 16 0 0.7842 -0.0026 6 16 1 -1.1780 0.0021 6 16 2 0.2140 -0.0012 6 16 3 -1.0187 -0.0049 6 16 4 -0.3265 -0.0008 6 17 0 0.8245 -0.0038 6 17 1 -0.4953 0.0027 6 17 2 0.9652 0.0017 6 17 3 0.1458 0.0013 6 17 4 0.5062 0.0078 6 18 0 0.4561 -0.0023 6 18 1 -0.6750 0.0025 6 18 2 0.1599 -0.0025 6 18 3 -0.5381 -0.0071 6 19 0 0.4011 -0.0042 6 19 1 -0.2057 0.0021 6 19 2 0.3322 0.0027 6 19 3 0.2384 0.0018 6 20 0 0.0883 -0.0003 6 20 1 0.0275 0.0011 6 20 2 -0.0518 -0.0023 6 20 3 -0.1105 -0.0059 6 21 0 -0.1242 -0.0018 6 21 1 0.0561 0.0006 6 21 2 -0.2059 0.0026 6 21 3 0.3025 0.0016 6 22 0 -0.0198 0.0015 6 22 1 0.5329 -0.0007 6 22 2 -0.1601 -0.0015 6 23 0 -0.4246 0.0007 6 23 1 0.0603 -0.0003 6 23 2 -0.3910 0.0017 6 24 0 0.1640 0.0013 6 24 1 0.5926 -0.0015 6 24 2 -0.0770 -0.0013 6 25 0 -0.3624 0.0014 6 25 1 -0.1366 0.0002 6 26 0 0.4137 -0.0007 6 26 1 0.2587 -0.0012 6 27 0 -0.0425 0.0006 6 27 1 -0.3073 0.0013 6 28 0 0.4925 -0.0025 6 28 1 -0.1912 -0.0003 6 29 0 0.2912 -0.0003 7 0 0 -0.8054 0.0044 7 0 2 0.2839 -0.0027 7 1 0 0.2525 -0.0023 7 1 1 0.1727 -0.0031 7 1 2 0.2400 0.0029 7 2 0 -0.7083 0.0027 7 2 1 -0.5235 -0.0001 7 2 2 0.3370 -0.0038 7 3 0 0.6060 -0.0046 7 3 1 0.0883 -0.0019 7 3 2 0.6367 0.0037 7 4 0 -0.5055 0.0016 7 4 1 -0.8128 -0.0007 7 4 2 0.4093 -0.0026 7 5 0 0.6284 -0.0049 7 5 1 0.0533 -0.0015 7 5 2 0.8252 0.0035 7 6 0 -0.3593 0.0017 7 6 1 -0.7967 -0.0013 7 6 2 0.3411 0.0007 7 7 0 0.4089 -0.0021 7 7 1 0.1661 -0.0022 7 7 2 0.7873 0.0019 7 8 0 -0.3202 0.0022 7 8 1 -0.6093 -0.0018 7 8 2 0.0864 0.0039 7 9 0 0.2263 0.0021 7 9 1 0.3556 -0.0030 7 9 2 0.6197 -0.0004 7 10 0 -0.2795 0.0023 7 10 1 -0.4783 -0.0018 7 10 2 -0.2254 0.0051 7 11 0 0.3121 0.0043 7 11 1 0.4443 -0.0028 7 11 2 0.4673 -0.0016 7 12 0 -0.1135 0.0012 7 12 1 -0.5397 -0.0012 7 12 2 -0.4154 0.0037 7 13 0 0.6505 0.0031 7 13 1 0.3363 -0.0011 7 13 2 0.4178 -0.0006 7 14 0 0.1589 -0.0009 7 14 1 -0.7266 -0.0006 7 14 2 -0.4227 0.0009 7 15 0 0.9834 -0.0002 7 15 1 0.1163 0.0014 7 15 2 0.4390 0.0021 7 16 0 0.3870 -0.0030 7 16 1 -0.8268 -0.0005 7 17 0 1.0157 -0.0028 7 17 1 -0.0433 0.0032 7 18 0 0.4452 -0.0037 7 18 1 -0.6677 -0.0009 7 19 0 0.6555 -0.0029 7 20 0 0.3486 -0.0028 0 0 0 0.0 0.0 ; _shelx_fab_checksum 21743 _olex2_submission_special_instructions 'No special instructions were received' _oxdiff_exptl_absorpt_empirical_details ; Empirical correction (ABSPACK) includes: - Absorption correction using spherical harmonics - Frame scaling ; _oxdiff_exptl_absorpt_empirical_full_max 1.399 _oxdiff_exptl_absorpt_empirical_full_min 0.802