If you try the nightly build (or 1.100 once it releases shortly) you’ll get a new Molecular Orbital Window
Now the one catch (since you show an open-shell species) is that it doesn’t yet handle separate alpha / beta spin orbitals. I wanted to make sure a bunch of other little pieces were fixed up before handling that. Extending the MO window to open-shell spieces is near the top of my list though.
But the basic idea would be a table of alpha and beta orbitals and you can click on whatever you want. By default orbitals +/- 5 from the HOMO / LUMO / SOMO would be generated.